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Pregled bibliografske jedinice broj: 984727

Highly Photostable and Fluorescent Microporous Solids Prepared via Solid-State Entrapment of Boron Dipyrromethene Dyes in a Nascent Metal–Organic Framework

Glembockyte, Viktorija; Frenette, Mathieu; Mottillo, Cristina; Durantini, Andres M.; Gostick, Jeff; Štrukil, Vjekoslav; Friščić, Tomislav; Cosa, Gonzalo
Highly Photostable and Fluorescent Microporous Solids Prepared via Solid-State Entrapment of Boron Dipyrromethene Dyes in a Nascent Metal–Organic Framework // Journal of the American Chemical Society, 140 (2018), 49; 16882-16887 doi:10.1021/jacs.8b09608 (međunarodna recenzija, prethodno priopćenje, znanstveni)

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Naslov
Highly Photostable and Fluorescent Microporous Solids Prepared via Solid-State Entrapment of Boron Dipyrromethene Dyes in a Nascent Metal–Organic Framework

Autori
Glembockyte, Viktorija ; Frenette, Mathieu ; Mottillo, Cristina ; Durantini, Andres M. ; Gostick, Jeff ; Štrukil, Vjekoslav ; Friščić, Tomislav ; Cosa, Gonzalo

Izvornik
Journal of the American Chemical Society (0002-7863) 140 (2018), 49; 16882-16887

Vrsta, podvrsta i kategorija rada
Radovi u časopisima, prethodno priopćenje, znanstveni

Ključne riječi
Fluorescent dyes ; metal-organic framework ; mechanochemistry

Sažetak
We report a strategy to synthesize highly emissive, photostable, microporous materials by solid-state entrapment of boron dipyrromethene (BODIPY) fluorophores in a metal–organic framework. Solvent-free mechanochemistry or accelerated aging enabled quantitative capture and dispersal of the PM605 dye within the ZIF-8 framework starting from inexpensive, commercial materials. While the design of emissive BODIPY solids is normally challenged by quenching in a densely packed environment, herein reported PM605@ZIF-8 materials show excellent emissive properties and to the best of our knowledge an unprecedented ∼10-fold enhancement of BODIPY photostability. Time-resolved and steady-state fluorescence studies of PM605@ZIF-8 show that interchromophore interactions are minimal at low dye loadings, but at higher ones lead to through-pore energy transfer between chromophores and to aggregate species.

Izvorni jezik
Engleski

Znanstvena područja
Kemija



POVEZANOST RADA

Ustanove:
Institut "Ruđer Bošković", Zagreb

Profili:

Avatar Url Vjekoslav Štrukil (autor)

Poveznice na cjeloviti tekst rada:

doi pubs.acs.org

Citiraj ovu publikaciju:

Glembockyte, Viktorija; Frenette, Mathieu; Mottillo, Cristina; Durantini, Andres M.; Gostick, Jeff; Štrukil, Vjekoslav; Friščić, Tomislav; Cosa, Gonzalo
Highly Photostable and Fluorescent Microporous Solids Prepared via Solid-State Entrapment of Boron Dipyrromethene Dyes in a Nascent Metal–Organic Framework // Journal of the American Chemical Society, 140 (2018), 49; 16882-16887 doi:10.1021/jacs.8b09608 (međunarodna recenzija, prethodno priopćenje, znanstveni)
Glembockyte, V., Frenette, M., Mottillo, C., Durantini, A., Gostick, J., Štrukil, V., Friščić, T. & Cosa, G. (2018) Highly Photostable and Fluorescent Microporous Solids Prepared via Solid-State Entrapment of Boron Dipyrromethene Dyes in a Nascent Metal–Organic Framework. Journal of the American Chemical Society, 140 (49), 16882-16887 doi:10.1021/jacs.8b09608.
@article{article, author = {Glembockyte, Viktorija and Frenette, Mathieu and Mottillo, Cristina and Durantini, Andres M. and Gostick, Jeff and \v{S}trukil, Vjekoslav and Fri\v{s}\v{c}i\'{c}, Tomislav and Cosa, Gonzalo}, year = {2018}, pages = {16882-16887}, DOI = {10.1021/jacs.8b09608}, keywords = {Fluorescent dyes, metal-organic framework, mechanochemistry}, journal = {Journal of the American Chemical Society}, doi = {10.1021/jacs.8b09608}, volume = {140}, number = {49}, issn = {0002-7863}, title = {Highly Photostable and Fluorescent Microporous Solids Prepared via Solid-State Entrapment of Boron Dipyrromethene Dyes in a Nascent Metal–Organic Framework}, keyword = {Fluorescent dyes, metal-organic framework, mechanochemistry} }
@article{article, author = {Glembockyte, Viktorija and Frenette, Mathieu and Mottillo, Cristina and Durantini, Andres M. and Gostick, Jeff and \v{S}trukil, Vjekoslav and Fri\v{s}\v{c}i\'{c}, Tomislav and Cosa, Gonzalo}, year = {2018}, pages = {16882-16887}, DOI = {10.1021/jacs.8b09608}, keywords = {Fluorescent dyes, metal-organic framework, mechanochemistry}, journal = {Journal of the American Chemical Society}, doi = {10.1021/jacs.8b09608}, volume = {140}, number = {49}, issn = {0002-7863}, title = {Highly Photostable and Fluorescent Microporous Solids Prepared via Solid-State Entrapment of Boron Dipyrromethene Dyes in a Nascent Metal–Organic Framework}, keyword = {Fluorescent dyes, metal-organic framework, mechanochemistry} }

Časopis indeksira:


  • Current Contents Connect (CCC)
  • Web of Science Core Collection (WoSCC)
    • Science Citation Index Expanded (SCI-EXP)
    • Arts & Humanities Citation Index (A&HCI)
    • SCI-EXP, SSCI i/ili A&HCI
  • Scopus
  • MEDLINE
  • Nature Index

Uključenost u ostale bibliografske baze podataka::


  • CA Search (Chemical Abstracts)
  • British Library
  • EBSCOhost
  • Ovid
  • Proquest
  • Thomson-Gale
  • SwetsWise

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