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Pregled bibliografske jedinice broj: 980969

Isotope Labeling Reveals Fast Atomic and Molecular Exchange in Mechanochemical Milling Reactions

Lukin, Stipe; Tireli, Martina; Stolar, Tomislav; Barišić, Dajana; Blanco, Maria Valeria; di Michiel, Marco; Užarević, Krunoslav; Halasz, Ivan
Isotope Labeling Reveals Fast Atomic and Molecular Exchange in Mechanochemical Milling Reactions // Journal of the American Chemical Society, 141 (2019), 3; 1212-1216 doi:10.1021/jacs.8b12149 (međunarodna recenzija, članak, znanstveni)

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Naslov
Isotope Labeling Reveals Fast Atomic and Molecular Exchange in Mechanochemical Milling Reactions

Autori
Lukin, Stipe ; Tireli, Martina ; Stolar, Tomislav ; Barišić, Dajana ; Blanco, Maria Valeria ; di Michiel, Marco ; Užarević, Krunoslav ; Halasz, Ivan

Izvornik
Journal of the American Chemical Society (0002-7863) 141 (2019), 3; 1212-1216

Vrsta, podvrsta i kategorija rada
Radovi u časopisima, članak, znanstveni

Ključne riječi
isotope labeling ; mechanochemistry ; mechanochemical deuteration ; in situ monitoring ; solid-state diffusion ; H/D exchange

Sažetak
Using tandem in situ monitoring and isotope- labeled solids, we reveal that mechanochemical ball-milling overcomes inherently slow solid- state diffusion through continuous comminution and growth of milled particles. This process occurs with or without a net chemical reaction and also occurs between solids and liquid additives that can be practically used for highly efficient deuterium labeling of solids. The presented findings reveal a fundamental aspect of milling reactions and also delineate a methodology that should be considered in the study of mechanochemical reaction mechanisms.

Izvorni jezik
Engleski

Znanstvena područja
Kemija



POVEZANOST RADA

Projekti:
HRZZ-UIP-2014-09-4744 - Mehanokemijska reaktivnost pod kontroliranim uvjetima temperature i atmosfere za čišću sintezu funkcionalnih materijala (MECHANOCONTROL) (Užarević, Krunoslav, HRZZ - 2014-09) ( CroRIS)

Ustanove:
Institut "Ruđer Bošković", Zagreb

Profili:

Avatar Url Ivan Halasz (autor)

Avatar Url Dajana Barišić (autor)

Avatar Url Tomislav Stolar (autor)

Avatar Url Martina Tireli (autor)

Avatar Url Stipe Lukin (autor)

Avatar Url Krunoslav Užarević (autor)

Poveznice na cjeloviti tekst rada:

doi pubs.acs.org www.doi.org

Citiraj ovu publikaciju:

Lukin, Stipe; Tireli, Martina; Stolar, Tomislav; Barišić, Dajana; Blanco, Maria Valeria; di Michiel, Marco; Užarević, Krunoslav; Halasz, Ivan
Isotope Labeling Reveals Fast Atomic and Molecular Exchange in Mechanochemical Milling Reactions // Journal of the American Chemical Society, 141 (2019), 3; 1212-1216 doi:10.1021/jacs.8b12149 (međunarodna recenzija, članak, znanstveni)
Lukin, S., Tireli, M., Stolar, T., Barišić, D., Blanco, M., di Michiel, M., Užarević, K. & Halasz, I. (2019) Isotope Labeling Reveals Fast Atomic and Molecular Exchange in Mechanochemical Milling Reactions. Journal of the American Chemical Society, 141 (3), 1212-1216 doi:10.1021/jacs.8b12149.
@article{article, author = {Lukin, Stipe and Tireli, Martina and Stolar, Tomislav and Bari\v{s}i\'{c}, Dajana and Blanco, Maria Valeria and di Michiel, Marco and U\v{z}arevi\'{c}, Krunoslav and Halasz, Ivan}, year = {2019}, pages = {1212-1216}, DOI = {10.1021/jacs.8b12149}, keywords = {isotope labeling, mechanochemistry, mechanochemical deuteration, in situ monitoring, solid-state diffusion, H/D exchange}, journal = {Journal of the American Chemical Society}, doi = {10.1021/jacs.8b12149}, volume = {141}, number = {3}, issn = {0002-7863}, title = {Isotope Labeling Reveals Fast Atomic and Molecular Exchange in Mechanochemical Milling Reactions}, keyword = {isotope labeling, mechanochemistry, mechanochemical deuteration, in situ monitoring, solid-state diffusion, H/D exchange} }
@article{article, author = {Lukin, Stipe and Tireli, Martina and Stolar, Tomislav and Bari\v{s}i\'{c}, Dajana and Blanco, Maria Valeria and di Michiel, Marco and U\v{z}arevi\'{c}, Krunoslav and Halasz, Ivan}, year = {2019}, pages = {1212-1216}, DOI = {10.1021/jacs.8b12149}, keywords = {isotope labeling, mechanochemistry, mechanochemical deuteration, in situ monitoring, solid-state diffusion, H/D exchange}, journal = {Journal of the American Chemical Society}, doi = {10.1021/jacs.8b12149}, volume = {141}, number = {3}, issn = {0002-7863}, title = {Isotope Labeling Reveals Fast Atomic and Molecular Exchange in Mechanochemical Milling Reactions}, keyword = {isotope labeling, mechanochemistry, mechanochemical deuteration, in situ monitoring, solid-state diffusion, H/D exchange} }

Časopis indeksira:


  • Current Contents Connect (CCC)
  • Web of Science Core Collection (WoSCC)
    • Science Citation Index Expanded (SCI-EXP)
    • SCI-EXP, SSCI i/ili A&HCI
  • Scopus
  • MEDLINE
  • Nature Index

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