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Thermal conductivity of (Ta1-xNbxSe4)2I alloys


Smontara, Ana; Lasjaunias, Jean, Claude; Maynard, Roger; Bilušić, Ante
Thermal conductivity of (Ta1-xNbxSe4)2I alloys // Proceedings of the Twenty-fourth International Thermal Conductivity Conference and Proceedings of the Twelfth International Thermal Expansion Symposium / Gaal, Peter S. ; Apostolescu, Daniela E. (ur.).
Lancaster: Technomic, 1999. str. 173-182 (pozvano predavanje, međunarodna recenzija, cjeloviti rad (in extenso), znanstveni)


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Naslov
Thermal conductivity of (Ta1-xNbxSe4)2I alloys

Autori
Smontara, Ana ; Lasjaunias, Jean, Claude ; Maynard, Roger ; Bilušić, Ante

Vrsta, podvrsta i kategorija rada
Radovi u zbornicima skupova, cjeloviti rad (in extenso), znanstveni

Izvornik
Proceedings of the Twenty-fourth International Thermal Conductivity Conference and Proceedings of the Twelfth International Thermal Expansion Symposium / Gaal, Peter S. ; Apostolescu, Daniela E. - Lancaster : Technomic, 1999, 173-182

ISBN
1-56676-711-3

Skup
International Thermal Conductivity Conference (24 ; 1999) ; International Thermal Expansion Symposium (12 ; 1999)

Mjesto i datum
Pittsburgh (PA), Sjedinjene Američke Države, 26.10.1997. - 29.10.1997

Vrsta sudjelovanja
Pozvano predavanje

Vrsta recenzije
Međunarodna recenzija

Ključne riječi
lattice thermal conductivtiy; lattice anharmonicity; quasi-one dimensional semiconductors

Sažetak
We present measurements and analysis of the phonon thermal conductivity k(T) of the alloys of the linear-chain compounds (TaSe4)2I and (Ta0.99Nb0.01Se4)2I, in the temperature range 60mK-6K. k(T) shows a very sharp peak in the vicinity of 1K and 2K for a (TaSe4)2I and (Ta0.99Nb0.01Se4)2I, respectively. The appearance of the peak in these systems is explained by a Poiseuille flow of phonons, originating from their strong anharmonicity amplified by the lattice anisotropy. k(T) of (TaSe4)2I obeys cubic variation (kľT3) below 0.8K, in good agreement with the boundary scattering regime. While k(T) of (Ta0.99Nb0.01Se4)2I and (TaSe4)2I (remeasured after a long storage at room temperature, and several thermal cycles down to 4K) in the temperature range 0.1K-1K and 60mK-6K, respectively, obeys quasi-quadratic regime (kľT1.8). This is ascribed to extended "linear or planar defects" specific to this very anisotropic structure, introduced either by doping Nb atoms in (TaSe4)2I or by successive thermal cycling. Below 0.1K, k(T) of (Ta0.99Nb0.01Se4)2I follows a cubic variation in good agreement with the boundary scattering regime.

Izvorni jezik
Engleski

Znanstvena područja
Fizika

Napomena
Predavač dr. sc. Ana Smontara.



POVEZANOST RADA


Projekti:
00350107

Ustanove:
Institut za fiziku, Zagreb

Profili:

Avatar Url Ana Smontara (autor)

Avatar Url Ante Bilušić (autor)

Citiraj ovu publikaciju:

Smontara, Ana; Lasjaunias, Jean, Claude; Maynard, Roger; Bilušić, Ante
Thermal conductivity of (Ta1-xNbxSe4)2I alloys // Proceedings of the Twenty-fourth International Thermal Conductivity Conference and Proceedings of the Twelfth International Thermal Expansion Symposium / Gaal, Peter S. ; Apostolescu, Daniela E. (ur.).
Lancaster: Technomic, 1999. str. 173-182 (pozvano predavanje, međunarodna recenzija, cjeloviti rad (in extenso), znanstveni)
Smontara, A., Lasjaunias, Jean, Claude, Maynard, R. & Bilušić, A. (1999) Thermal conductivity of (Ta1-xNbxSe4)2I alloys. U: Gaal, P. & Apostolescu, D. (ur.)Proceedings of the Twenty-fourth International Thermal Conductivity Conference and Proceedings of the Twelfth International Thermal Expansion Symposium.
@article{article, author = {Smontara, Ana and Maynard, Roger and Bilu\v{s}i\'{c}, Ante}, year = {1999}, pages = {173-182}, keywords = {lattice thermal conductivtiy, lattice anharmonicity, quasi-one dimensional semiconductors}, isbn = {1-56676-711-3}, title = {Thermal conductivity of (Ta1-xNbxSe4)2I alloys}, keyword = {lattice thermal conductivtiy, lattice anharmonicity, quasi-one dimensional semiconductors}, publisher = {Technomic}, publisherplace = {Pittsburgh (PA), Sjedinjene Ameri\v{c}ke Dr\v{z}ave} }
@article{article, author = {Smontara, Ana and Maynard, Roger and Bilu\v{s}i\'{c}, Ante}, year = {1999}, pages = {173-182}, keywords = {lattice thermal conductivtiy, lattice anharmonicity, quasi-one dimensional semiconductors}, isbn = {1-56676-711-3}, title = {Thermal conductivity of (Ta1-xNbxSe4)2I alloys}, keyword = {lattice thermal conductivtiy, lattice anharmonicity, quasi-one dimensional semiconductors}, publisher = {Technomic}, publisherplace = {Pittsburgh (PA), Sjedinjene Ameri\v{c}ke Dr\v{z}ave} }




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