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Pregled bibliografske jedinice broj: 780731

Ligandless Iron-catalyzed Desulfinylative C-C Allylation reactions using Grignard reagents and Alk-2-enesulfonyl Chlorides

Volla, C. M. R.; Markovic, D.; Dubbaka S. R.; Vogel, P.
Ligandless Iron-catalyzed Desulfinylative C-C Allylation reactions using Grignard reagents and Alk-2-enesulfonyl Chlorides // European journal of organic chemistry, 36 (2009), 6281-6288 doi:10.1002/ejoc.200900927 (međunarodna recenzija, članak, znanstveni)

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Naslov
Ligandless Iron-catalyzed Desulfinylative C-C Allylation reactions using Grignard reagents and Alk-2-enesulfonyl Chlorides

Autori
Volla, C. M. R. ; Markovic, D. ; Dubbaka S. R. ; Vogel, P.

Izvornik
European journal of organic chemistry (1434-193X) 36 (2009); 6281-6288

Vrsta, podvrsta i kategorija rada
Radovi u časopisima, članak, znanstveni

Ključne riječi
Desulfinylative C-C allylation reactions; Grignard reagents; Alk-2-enesulfonyl Chlorides

Sažetak
Alk-2-enesulfonyl chlorides 1–4 were synthesized by the BCl3-promoted ene reaction of alkenes with SO2. These sulfonyl chlorides were then used as electrophilic partners in iron-catalyzed desulfinylative cross-coupling reactions with different Grignard reagents (aromatic, aliphatic, andheteroaromatic). The reaction can be catalyzed with even 2 mol-% of the simple iron salt Fe(acac)3. The regioselectivity of these allylations was studied by using sulfonyl chlorides 3 and 4 with aryl Grignard reagents. The scope of these allylations was further extended by the coupling of ester-substituted alk-2-enesulfonyl chloride 10 with aromatic Grignard reagents. Symmetrical products were synthesized by double C–C allylation with the use of 2-methylidenepropane-1, 3-disulfonyl chloride (12).

Izvorni jezik
Engleski

Znanstvena područja
Kemija



POVEZANOST RADA

Profili:

Avatar Url Dean Marković (autor)

Poveznice na cjeloviti tekst rada:

doi onlinelibrary.wiley.com

Citiraj ovu publikaciju:

Volla, C. M. R.; Markovic, D.; Dubbaka S. R.; Vogel, P.
Ligandless Iron-catalyzed Desulfinylative C-C Allylation reactions using Grignard reagents and Alk-2-enesulfonyl Chlorides // European journal of organic chemistry, 36 (2009), 6281-6288 doi:10.1002/ejoc.200900927 (međunarodna recenzija, članak, znanstveni)
Volla, C., Markovic, D., Dubbaka S. R. & Vogel, P. (2009) Ligandless Iron-catalyzed Desulfinylative C-C Allylation reactions using Grignard reagents and Alk-2-enesulfonyl Chlorides. European journal of organic chemistry, 36, 6281-6288 doi:10.1002/ejoc.200900927.
@article{article, author = {Volla, C. M. R. and Markovic, D. and Vogel, P.}, year = {2009}, pages = {6281-6288}, DOI = {10.1002/ejoc.200900927}, keywords = {Desulfinylative C-C allylation reactions, Grignard reagents, Alk-2-enesulfonyl Chlorides}, journal = {European journal of organic chemistry}, doi = {10.1002/ejoc.200900927}, volume = {36}, issn = {1434-193X}, title = {Ligandless Iron-catalyzed Desulfinylative C-C Allylation reactions using Grignard reagents and Alk-2-enesulfonyl Chlorides}, keyword = {Desulfinylative C-C allylation reactions, Grignard reagents, Alk-2-enesulfonyl Chlorides} }
@article{article, author = {Volla, C. M. R. and Markovic, D. and Vogel, P.}, year = {2009}, pages = {6281-6288}, DOI = {10.1002/ejoc.200900927}, keywords = {Desulfinylative C-C allylation reactions, Grignard reagents, Alk-2-enesulfonyl Chlorides}, journal = {European journal of organic chemistry}, doi = {10.1002/ejoc.200900927}, volume = {36}, issn = {1434-193X}, title = {Ligandless Iron-catalyzed Desulfinylative C-C Allylation reactions using Grignard reagents and Alk-2-enesulfonyl Chlorides}, keyword = {Desulfinylative C-C allylation reactions, Grignard reagents, Alk-2-enesulfonyl Chlorides} }

Časopis indeksira:


  • Current Contents Connect (CCC)
  • Web of Science Core Collection (WoSCC)
    • Science Citation Index Expanded (SCI-EXP)
    • SCI-EXP, SSCI i/ili A&HCI
  • Scopus

Uključenost u ostale bibliografske baze podataka::


  • Desulfinylative C-C allylation reactions, Grignard reagents, Alk-2-enesulfonyl Chlorides

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