ÐÏà¡±á>þÿ ½¿þÿÿÿ»¼Á<=>¸sýpÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿÿì¥Áq`ø¿ªNbjbjqPqP BX::ê;%ÿÿÿÿÿÿ¤ììììœœœ°\t\t\t8”täxv°h§b˜x‚y"W},†ƒ}$§}}}}¦¦2†^}}}h§¬~¬~¬~¬~°°$ÔD5ED/°°ÔE°°°ììììììÿÿÿÿSIMULATION AND ANALYSIS OF POST-COMBUSTION CO2 CAPTURE BY ABSORPTION Lj.MATIJA`EVI1, I.DEJANOVI1 and G.KOVAI2 1 Faculty of Chemical Engineering and Technology, University of Zagreb,Savska c.16, 10000 Zagreb, Croatia, 2 EKONERG - Energy and Environmental Protection Institute, Koranska 5, 10000 Zagreb, Croatia e-mail: ljmatij@fkit.hr EXTENDED ABSTRACT This paper presents an analysis of a system for CO2 capture from a power plant's flue gas by chemical absorption in aqueous monoethanolamine (MEA), which has previously been commercially applied to systems with smaller capacity. The process of CO2 capture by absorption, together with the facility for the compression of separated CO2, was modelled in ChemCAD process simulator. Based on simulations, best operating conditions were chosen. Equipment sizing and assessment of investment and operating costs were also carried out, and based on that data cost-effectiveness analysis of the plant was made. This system for CO2 capture is a part of a new power block which will be built on the site of an existing local power plant. In this work is shown that CO2 capture technology is very energy and capital intensive and that its implementation reduces the energy efficiency of the power plant by almost 10 %. Also, this system requires up to 50% increase in cooling water use. Because of significant capital cost and great parasitic effect on power plant net electrical capacity, 50% increase of electricity cost was estimated in the case of this capture system application. The cost of CO2 avoided for power plant with CO2 capture system installed (only capture plant) was estimated to 38.5 ¬ /t CO2. This is the value that determines the emission units price at which this system would be cost effective. If this system would be subsequently retrofitted (which is more likely) the price would be even higher, and for the entire CCS system, which includes transport and geological storage of captured CO2, the price value could reach and outgrow 50 ¬ /t CO2. Keywords: power plant, carbon capture, carbon dioxide, chemical absorption 1. INTRODUCTION Coal has been used as a power plant fuel for decades, and today its share in global electricity production is around 42% compared to other energy sources (natural gas, liquid fuels, nuclear fuels and renewable energy sources Figure 1 illustrates energy sources in electricity production in the world in 2007., according to data from the Energy Information Administration (EIA) [1]. Figure1.Percentage of coal in electricity production in the world The advantage of coal as a fuel is in its price, i.e., coal is the cheapest source of energy in energy production. The low price partly compensates high investment costs of coal power plants [2]. Despite many advantages, the biggest drawback of using coal is the increased pollution of the environment, primarily through air emissions of various pollutants, compared to power plants that use natural gas and especially to those running on renewable energy sources. Combustion of coal in relation to the competitive fossil fuel - natural gas, produces far more carbon dioxide, which is the most common greenhouse gas. New technologies of coal combustion, so-called clean coal technologies, together with conventional end-of-pipe solutions, enable far lower emissions of air pollutants (sulphur and nitrogen oxides, particulates, heavy metals) by using different systems for their effective removal from flue gases, and also lead to significant reduction in carbon dioxide emissions [3,4,5]. This paper presents an analysis of a system for CO2 capture from a power plant flue gas by chemical absorption in aqueous monoethanolamine (MEA), which has previously been commercially applied to systems with smaller capacity. Good review about post-combustion CO2 capture with chemical absorption is given by Wang M. et al. [6]. Review of recent literature showed that CCS systems modelling and optimisation is an important research field [7, 8, 9, 10] and that there is a lot of issues to be solved for successful and sustainable application of carbon capture technologies. 2. ANALYSIS AND CALCULATION OF CO2 CAPTURE SYSTEM 2.1. Parameters of the reference power plant The planned electric generation capacity of the plant is 500 MW gross, with supercritical CO2 generation and very low emissions of pollutants. Basic parameters of the power plant are shown in Table 1 and characteristics of flue gas in Table 2. Table 1: Basic parameters unitvalueCoalfuel consumptionkg/s39.69t/h142.88lower heating valueMJ/kg26.3heat entered with fuelMJ/s (MWt)1044PowergeneratorMW500own consumptionMW25.34%5.07net powerMW474.66Efficiencygenerator%47.9net (threshold of power)%45.47 Table 2: Characteristics of flue gases unitvaluemass flow rate of flue gaseskg/s495.18pressurekPa101.60temperature°C50compositionN2% mass69.52H2O (g)% mass6.34CO2% mass19.29O2% mass4.85 2.2 Simulation of CO2 capture system MEA absorption system was modelled in ChemCAD, using following assumptions: the cooling sea water has inlet temperature of 15°C, with allowable increase of 8-9°C; absorption has to remove 90% of total CO2; aqueous MEA solution is 30% by weight; purity of CO2 after the stripper column is 98 %. The process was modelled in three distinctive parts, using appropriate thermodynamic models. The distinctive parts were flue gas cooling and absorption/regeneration, shown in Figure 2, and CO2 compression, shown in Figure 3. Absorber and stripper columns were modelled using SCDS module in ChemCAD, with 12 and 20 equilibrium stages respectively. Absorption column is operated at atmospheric pressure (1 bar). Water wash, at 25°C, is fed into the column at the top stage, while lean amine solution, at 40°C, is introduced at 4th stage. Rich amine solution, preheated to 105°C, is fed into the stripper column at 2nd stage. Column top pressure is 1.7 bar, and estimated pressure drop 0.3 bar. In order to get necessary CO2 purity at the top, partial condenser outlet temperature was set to 40°C, while reboiler specification was varied to obtain required lean amine composition (mol CO2/mol MEA). Lean amine recirculation is used to preheat column feed, and then cooled in a trimmer cooler to 40°C. Water balance in the model was maintained using controller module in feed-back mode, used to adjust water wash flow rate. EMBED Visio.Drawing.11 Figure 2: Process flow diagram for CO2 capture by chemical absorption Compression of captured CO2 was modelled as four-stage compression with intercoolers, which cool compressed gas to 40°C. The pressure ratio in first three compressors was set to 3, and in the last compressor to 2, with efficiency of 75%. After first 3 intercoolers, condensed water was separated using flash drums, resulting in CO2 purity of 99.99 mol. %. After last compressor supercritical CO2 was cooled to 25°C, and pumped to the final required pressure of 110 bar. EMBED Visio.Drawing.11 Figure 3: Process flow diagram of CO2 compression 2.3 Results and discussion Parametric study The main operating parameter of the CO2 capture system is the lean amine solution load (±LEAN), which is the remaining absorbed CO2 to MEA molar ratio. To determine the optimal value, its influence on four different process variables was performed: required flow rate of wash water (Fig.4), MEA use (Fig.5), total cooling heat duty (Fig.6) and heat duty of the reboiler (Fig.7). The results show that increase of remaining CO2 to MEA ratio in the lean amine solution (±LEAN) leads to decrease in water wash flow rate, i.e. reduction of lost water (as shown in Figure 4), which can be explained with reduction of specific heat generated by reaction between MEA and CO2. The increase in ±LEAN causes increase in the amount of MEA required for 90% removal of CO2, as shown in Figure 5. This is due to decrease of MEA capacity to bound CO2 from the flue gas, caused by CO2 remaining in the solution. EMBED SigmaPlotGraphicObject.10 EMBED SigmaPlotGraphicObject.10 Figure 4. Water wash use use versus Figure 5. MEA use versus MEA load MEA load EMBED SigmaPlotGraphicObject.10 EMBED SigmaPlotGraphicObject.10 Figure 6. Total cooling heat duty versus Figure 7. Heat duty of reboiler versus MEA load MEA load Total cooling heat duty (the sum of heat duties of lean amine cooler and stripper column's condenser) increases for low values of ±LEAN, because of increase of the vapour load in the stripper column, leading to higher condenser duty. It also increases for higher values of ±LEAN because of increase of the lean amine flow rate in lean amine cooler. Due to this trade-off, there is a minimum of total cooling heat duty at ±LEAN values between 0.15 0.19 mol CO2/mol MEA. Reboiler heat duty values were between 3.4 3.5 GJ/t CO2 for most of ±LEAN values, with significant increase (> 4.0 GJ/t CO2) at lower values. This can be explained with larger amount of heat required for dissociation of CO2 and MEA molecules, and larger amount of water that needs to be evaporated for CO2 stripping. At higher ±LEAN values, heat required for dissociation and evaporation is reduced, but the heat duty also increases because of larger rich amine flow rates. These heat duty values are in agreement with values in other studies, where reboiler duties were reported to be between 3.2 – 4.0 GJ/ t CO2 [11]. Due to lower flow rate of recirculating MEA solution required for 90% absorption (value directly influencing equipment size and capital costs), lower cooling water flow rate and lower reboiler heat duties, an ±LEAN value for detailed dimensioning and economic analysis was taken to be 0.184 mol CO2/mol MEA. Sizing and economical assessment There is still relatively little reported experience with all three components of this system: capture, transport and storage of CO2 in a fully integrated CCS system. In this work detailed design was not carried out. As in other reported studies, certain assumptions that may affect the cost estimates were made. Absorption and stripper columns were equipped with structured packing Montz-Pak B1-200. The dimensions of absorber and stripper column were determined using structured packing sizing tool in ChemCAD, requiring specification of HETP values, with maximum allowable flooding below 80%. Results are shown in Table 3. Table 3: Dimensions of absorber and stripper column ABSORBERSECTION (water wash)diameter (m)12.0height (m)8.0SECTION (absorption)diameter (m)16.6height (m)29.0STRIPPERENTIRE COLUMNdiameter (m)8.6height (m)17.0 Estimation of capital equipment cost was performed using ChemCAD costing tool. Column costs include shells with internal equipment (packing, distributors, collectors and support grids). Reboiler and condenser costs were added to total heat exchanger costs. The costs of produced electricity and avoided CO2, with and without CCS, are reported in Table 4, utilities' use in Table 5, while influence of CCS implementation on power plants' output in Table 6. Table 4: Overall annual cost with costs electricity and avoided CO2 UNITPOWERPOWER + CCSCapital cost106 US$9751236Operating cost106 US$/year25.941.9Fuel cost106 US$/ year115.9115.9Annual capital cost106 US$/ year92.8117.6Overall annual cost106 US$/ year234.6275.4Electricity producedMWh/ year3,607,720.02,847,872.0Specific emissions of CO2t/MWh0.7250.092Electricity costUS$/MWh65.0296.70Cost avoided CO2US$/t CO250.1Cost avoided CO2¬ /t CO238.5 Cost avoided CO2 is defined by Eq.(1), where ref is reference plant and ccs is plat with CCS. EMBED Equation.3 (1) Table 5. 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sH Ï@#A$A%A*A0ADQDRDSDTDaDdDéÔ¿¬¿š…¿}ncP?n4ÔhŸshL&8mH sH !j³±hŸshPg°EHÞÿUmH sH %jÆV)))$$„üÿ„&`#$/„´Ifa$gd³µÁkd×¹$$If–l4ÖÖ\”ÿ˜(|à€ €T€ tà 6`”üÿ””´Ö0ÿÿÿÿÿÿöˆ6ööÖÿÿÿÿÖÿÿÿÿÖÿÿÿÿÖÿÿÿÿ”´4Ö4Ö laöpÖ(ÿÿÿÿÿÿÿÿ 50 ¬ /t . This means that this CSS system would be economically feasible if cost of emission units would be higher. Price of emission units, however, is difficult to predict and current expected values lie between 20 40 ¬ /t CO2. Many open questions related to safety and ecological as well as economical sustainability of CCS system application should be resolved before its implementation in a power plant. REFERENCES IEA (2009), Key world Energy statistics, Kaplan S. (2008), Power Plants:Charasteristics and Costs, Congressional Research service Report RL34746, Michigan Minchener A.J., McMullan J.T. (2007), Significant achievements of European Coal and Steel community R&D programmes in the development of clean coal power generation technology, IEA Coal Research Ltd. 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(2010), Modelling reactive absorption of CO2 in packed columns for post combustion carbon capture applications, Chem.Eng.Res.Des., doi:101016/j.cherd.2010.09.0020 ,,`,d,p,aXLL$$Ifa$gd;4, $Ifgd;4,žkd¢½$$If–lÖÖFpGì!€×€¥€Á tàÖ0ÿÿÿÿÿÿö6ööÖÿÿÿÖÿÿÿÖÿÿÿÖÿÿÿ4Ö4Ö laöÜpÖÿÿÿÿÿÿp,r,Î,Ò,Ü,aXLL$$Ifa$gd;4, $Ifgd;4,žkdC¾$$If–lÖÖFpGì!€×€¥€Á tàÖ0ÿÿÿÿÿÿö6ööÖÿÿÿÖÿÿÿÖÿÿÿÖÿÿÿ4Ö4Ö laöÜpÖÿÿÿÿÿÿÜ,Þ,ü, --aXLL$$Ifa$gd;4, $Ifgd;4,žkdä¾$$If–lÖÖFpGì!€×€¥€Á tàÖ0ÿÿÿÿÿÿö6ööÖÿÿÿÖÿÿÿÖÿÿÿÖÿÿÿ4Ö4Ö laöÜpÖÿÿÿÿÿÿü,--- ------4-6-:-<-B-D-H-J-P-R-T-V-t-v-ø-....%.U.éÒé½éÒé½é½éÒé½éÒé½ˆxcNcNcNc(h>èhECJOJQJ^JaJmH sH (h>èh’/CJOJQJ^JaJmH sH h>èhË„5CJOJQJ^J(hŸshË„5B*CJOJQJ^JphhntÕh³µ5CJOJQJ^JhntÕhq5CJ,aJ,mH sH (h•c`hqCJOJQJ^JaJmH sH ,h•c`hÓh(CJOJPJQJ^JaJmH sH ,h•c`hqCJOJPJQJ^JaJmH sH --6-D-R-aXLL$$Ifa$gd;4, $Ifgd;4,žkd…¿$$If–lÖÖFpGì!€×€¥€Á tàÖ0ÿÿÿÿÿÿö6ööÖÿÿÿÖÿÿÿÖÿÿÿÖÿÿÿ4Ö4Ö laöÜpÖÿÿÿÿÿÿR-T-V-t-v-q.h0ô2a_U_IAI$a$gdöeØ$7$8$H$a$gd¾b. 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