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lvana Novak Original scientific paperDepartment of Applied Chemistry and Ecology, Faculty of Food Technology, University of Josip JurajStrossmayer, Kuhadeva 18, 31000 Osijek, Croatia, (e-mail: ljakobek@ptfos.hr) AbstractTotal polr,phenols (TP), total anthocvanins (TA) and antioxidant activitv of various fruits (black currant, redcurrant, sour cherry, elderberrv, arrd blueberry) were determined bv using Folin-Ciocalteau, pH-differential andDPPH n'rethod. In order to identifu individual non-anthocvanic phenolic compounds fflavonols (quercetin,tlvricetin, kaempferol), phenolic acids (p-coumaric, caffeic, ferulic, p-hvdron,benzoic and ellagic acid)] presentin chosen fruits, HPLC method r,vas applied. The highest amounts of TP and TA, and the strongest antioxidantactivities lvere found in blueberr-v, elderberrv and black currant. The major non-anthocvanic phenoliccomPonent in elderberrv and blueberrv was quercetin. In black currant, myricetin vvas the most abundantphenolic compound. P-hvdroxvbenzoic acid rvas the main phenolic compound of red currant, whereas p-coumaric and caffeic acid were the most abundant phenolic compounds of sour cherrv.Key words: anthocyanins, berry fruit, flavonols, phenolic acidslntroductionPolrphenolic compounds, like flavonols, anthocyanins and phenolic acids, are important components of fruitsr\lAAtti-Riihinen et al.,2004). Thev are studied intensivelv because of possible beneficial effects on humanhealth (Beattie et al., 2005). Po\phenolic compounds possess antioxidant activitv in vitro (K.Jhkonen et al.,2003) and mav be protective against manv degenerative diseases (lGekt et al., 2002). There is still not enoughknou4edge about health effects of fruits and their polr,phenols and much more research is, therefore, needed,ru the composition of polvphenolic antioxidants in fruits and on antioxidant effects of fruits (Heinonen et.r1., 2002). The objective of this rvork l'vas to evaluate some fruits (black currant, red currant, sour cherry,clderberrv and blueberry) regarding the amount of total pol.nphenols, total anthocvanins and antioxidantectivitv and to identifu individual flavonols (quercetin, kaempferol and mvricetin) and phenolic acids (p-coumaric, caffeic, ferulic, p-hvdroxvbenzoic and ellagic acid) present in these fruits.Materials and methodsChemicals-l-hvdrorrybenzoic acid, ellagic acid, caffeic acid, ferulic acid, p-coumaric acid, mwicetin, quercetin dihydrate,kaempferol, 2,2-diphenyl-l-picrvlhvdrazvl radical (DPPH),'uvere purchased from Sigma-Aldrich (St. Louis,\1O, USA). Methanol (HPLC grade) was obtained from Merck (Darmstadt, Germanv) and ortho-phosphoricacid (B5o/o, HPLC grade) rvas purchased from Fluka (Buchs, Switzerland). Hydrochloric acid (36.2 o/o),potassium chloride, sodium acetate trihvdrate, Folin-Ciocalteau reagent were obtained from IGmika (Zagreb,Croatia). Determination of total polr,nhenols, total anthocvanins and antioxidant activityFruits fblack currant (fubes nigrum), red currant (fubes satir.um), sour cherrv (Prunus cerasus), elderberrv(Sambucus nigra), blueberrv (Vaccinium sp.)] were harvested in Slavonia region (Croatia), frozen and stored''irf 'l*i*,Al'l & :rI iilll:nliATl*liAl $Yl,,1p*$llf,l *ll A*tllilLlUq: I 633 endstream endobj 7 0 obj 3359 endobj 8 0 obj << /Length 27 >> stream % CANON_PFINF_TYPE0_TEXTON endstream endobj 9 0 obj << /Length 44 >> stream q 597.12 0 0 835.20 0.00 0.00 cm /Obj2 Do Q endstream endobj 10 0 obj << /Type /Page /MediaBox [ 0 0 597.12 835.20 ] /Parent 11 0 R /Resources << /Font << /F3 5 0 R >> /XObject << /Obj2 2 0 R >> /Subtype 6 0 R /ProcSet [ /PDF /Text /ImageB /ImageC /ImageI ] >> /Contents [ 8 0 R 9 0 R 3 0 R ] >> endobj 13 0 obj << /Type /XObject /Subtype /Image /Width 2488 /Height 3480 /BitsPerComponent 1 /ColorSpace /DeviceGray /Filter /CCITTFaxDecode /DecodeParms << /K -1 /Columns 2488 >> /Length 96908 >> stream +Dwu2HUP@|Gĺ@@qK#ؑ_@>CyV#GT##(/˨&8"; ~ Cae@ i^aaAp@U;)# Dt]i1#AYP'ۈp?{#B<è/GTCTPGz((uyC{2:u{Et]Et]D|"G A$L)98qK(xЋ #|>G㈈)$q&=q98rc>CDXBa2>#|>G0^<Ɏ)9C㤑8sLs}Pd|>GyCsLp@DDD_It9Hsq98pǡDZ!d|S9&>")$#%q8sq9 x!a4">CCDD0Hc8sq98".hpD9qG2:G#|>G#|I$H$QɎqDDEP8L&G#|>Gq"""""A$88918 8B!d|>G#|yHRI$dI#Lsqs"""({ L>G#|:qDDDDRI&EGrc8ELd|#s#P8,DDDDE D~I$988p@a8GL&Gl>G2>Grc!I#G#q98""""a0 9C:sEDDDZWBGq98sq8(u)9C:a(sLsq8CDI$98sq9|u"""-4Exa Crq}: Gt98sq#WI "rnPꄐP$8A2>G#|"P"""I$I8Dt7g89nqqDuB,#&G#|&GL:8I I$A:."9)98"""(B"!& >G#|?sqIHRI#q9898L! &##|98p@DDRuI$H$)E9)rTC_? 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0 1 400.80 559.68 Tm <6163744D747920> Tj 1 0 0 1 434.64 560.16 Tm <7276617320> Tj 1 0 0 1 453.84 560.64 Tm <64657465726D696E656420> Tj 1 0 0 1 505.20 561.36 Tm <7573696E67> Tj 0.48 Tc 1 0 0 1 68.88 539.28 Tm <74686520> Tj 1 0 0 1 85.92 539.76 Tm <322C322D64697068656E766C2D492D70696372796C68766472617A766C20> Tj 1 0 0 1 215.28 542.40 Tm <28445050482920> Tj 1 0 0 1 253.44 542.40 Tm <6D6574686F6420> Tj 1 0 0 1 289.92 543.36 Tm <2842656E76656E75746920> Tj 1 0 0 1 339.36 543.60 Tm <657420> Tj 1 0 0 1 350.88 543.84 Tm <616C2E2C20> Tj 1 0 0 1 366.48 544.32 Tm <32303034292E20> Tj 1 0 0 1 397.92 544.80 Tm <546872656520> Tj 1 0 0 1 426.00 545.04 Tm <6F7220> Tj 1 0 0 1 438.24 545.28 Tm <6669766520> Tj 1 0 0 1 456.72 545.76 Tm <64696C7574696F6E7320> Tj 1 0 0 1 497.04 546.24 Tm <6F6620> Tj 1 0 0 1 508.56 546.48 Tm <65616368> Tj 0.24 Tc 1 0 0 1 69.12 524.88 Tm <667275697420> Tj 1 0 0 1 90.72 524.88 Tm <6578747261637420> Tj 1 0 0 1 121.68 525.60 Tm <7765726520> Tj 1 0 0 1 144.48 525.84 Tm <616E616C767A65642E20> Tj 1 0 0 1 187.20 526.56 Tm <5265616374696F6E20> Tj 1 0 0 1 227.28 527.04 Tm <736F6C7574696F6E20> Tj 1 0 0 1 264.00 527.76 Tm <7276617320> Tj 1 0 0 1 282.72 527.76 Tm <707265706172656420> Tj 1 0 0 1 322.32 528.48 Tm <627920> Tj 1 0 0 1 336.00 528.96 Tm <6D6C78696E6720> Tj 1 0 0 1 367.68 529.20 Tm <353020> Tj 1 0 0 1 381.60 530.16 Tm <706C20> Tj 1 0 0 1 392.64 529.68 Tm <6F6620> Tj 1 0 0 1 403.92 529.92 Tm <64696C7574656420> Tj 1 0 0 1 436.80 530.40 Tm <667275697420> Tj 1 0 0 1 458.16 530.88 Tm <6578747261637420> Tj 1 0 0 1 489.12 531.36 Tm <6C7669746820> Tj 1 0 0 1 511.44 531.60 Tm <333030> Tj 0.48 Tc 1 0 0 1 69.60 510.48 Tm <706C20> Tj 1 0 0 1 80.40 510.24 Tm <6F6620> Tj 1 0 0 1 91.92 510.48 Tm <6D657468616E6F6C696320> Tj 1 0 0 1 141.60 511.20 Tm <4450504820> Tj 1 0 0 1 174.24 511.68 Tm <736F6C7574696F6E20> Tj 1 0 0 1 211.92 512.64 Tm <28496D4D2920> Tj 1 0 0 1 245.28 512.88 Tm <616E6420> Tj 1 0 0 1 263.76 513.12 Tm <62726F7567687420> Tj 1 0 0 1 299.76 513.60 Tm <746F20> Tj 1 0 0 1 311.76 513.84 Tm <3320> Tj 1 0 0 1 320.16 514.08 Tm <6D6C20> Tj 1 0 0 1 333.60 514.08 Tm <727669746820> Tj 1 0 0 1 355.68 514.56 Tm <6D657468616E6F6C2E20> Tj 1 0 0 1 401.04 515.52 Tm <54686520> Tj 1 0 0 1 421.20 515.52 Tm <736F6C7574696F6E20> Tj 1 0 0 1 457.68 516.24 Tm <77617320> Tj 1 0 0 1 476.40 516.48 Tm <6B65707420> Tj 1 0 0 1 498.00 516.96 Tm <696E20> Tj 1 0 0 1 509.28 516.96 Tm <6461726B> Tj 0.48 Tc 1 0 0 1 69.84 495.60 Tm <617420> Tj 1 0 0 1 80.40 495.84 Tm <726F6F6D20> Tj 1 0 0 1 105.12 496.08 Tm <74656D706572617475726520> Tj 1 0 0 1 159.36 497.04 Tm <666F7220> Tj 1 0 0 1 174.96 497.28 Tm <6C3520> Tj 1 0 0 1 187.44 497.52 Tm <6D696E757465732E20> Tj 1 0 0 1 226.32 498.00 Tm <54686520> Tj 1 0 0 1 246.00 498.24 Tm <6162736F7262616E636520> Tj 1 0 0 1 296.16 499.44 Tm <284122222E222E2920> Tj 1 0 0 1 328.56 499.68 Tm <5C6C27617320> Tj 1 0 0 1 347.28 499.92 Tm <7265616420> Tj 1 0 0 1 367.92 500.16 Tm <616761696E737420> Tj 1 0 0 1 400.08 500.64 Tm <74686520> Tj 1 0 0 1 416.16 500.88 Tm <707265706172656420> Tj 1 0 0 1 455.52 501.84 Tm <626C616E6B20> Tj 1 0 0 1 482.16 502.08 Tm <617420> Tj 1 0 0 1 492.96 502.08 Tm <35313720> Tj 1 0 0 1 511.92 502.56 Tm <6E6D27> Tj 0.48 Tc 1 0 0 1 69.60 480.96 Tm <54686520> Tj 1 0 0 1 89.76 481.20 Tm <6162736F7262616E636520> Tj 1 0 0 1 140.16 482.40 Tm <28412C2C2C6F6F6E2920> Tj 1 0 0 1 172.80 482.64 Tm <6F6620> Tj 1 0 0 1 184.32 482.88 Tm <4450504820> Tj 1 0 0 1 216.48 483.12 Tm <626C616E6B20> Tj 1 0 0 1 243.36 483.60 Tm <736F6C7574696F6E20> Tj 1 0 0 1 280.80 484.56 Tm <2833303020> Tj 1 0 0 1 303.84 485.04 Tm <706C20> Tj 1 0 0 1 314.64 484.80 Tm <6F6620> Tj 1 0 0 1 327.36 485.04 Tm <6C6D4D20> Tj 1 0 0 1 352.80 485.28 Tm <4450504820> Tj 1 0 0 1 385.44 486.00 Tm <736F6C7574696F6E2C20> Tj 1 0 0 1 425.04 486.48 Tm <32273720> Tj 1 0 0 1 441.60 486.96 Tm <6D6C20> Tj 1 0 0 1 455.28 486.96 Tm <6F6620> Tj 1 0 0 1 466.80 487.20 Tm <6D657468616E6F6C2920> Tj 1 0 0 1 513.12 487.92 Tm <776173> Tj 0.24 Tc 1 0 0 1 70.32 466.32 Tm <6D6561737572656420> Tj 1 0 0 1 113.04 466.80 Tm <6461696C792E20> Tj 1 0 0 1 137.76 469.92 Tm <70657263656E7420> Tj 1 0 0 1 171.36 467.76 Tm <696E6869626974696F6E20> Tj 1 0 0 1 216.00 468.48 Tm <6F6620> Tj 1 0 0 1 227.28 468.72 Tm <4450504820> Tj 1 0 0 1 258.00 469.20 Tm <7261646963616C20> Tj 1 0 0 1 288.72 469.68 Tm <722776617320> Tj 1 0 0 1 307.20 469.68 Tm <63616963756C6174656420> Tj 1 0 0 1 352.08 470.64 Tm <666F7220> Tj 1 0 0 1 366.72 470.88 Tm <6561636820> Tj 1 0 0 1 388.80 471.12 Tm <64696C7574696F6E20> Tj 1 0 0 1 425.04 471.84 Tm <6F6620> Tj 1 0 0 1 436.32 472.08 Tm <667275697420> Tj 1 0 0 1 457.44 472.32 Tm <6578747261637420> Tj 1 0 0 1 488.88 472.80 Tm <6163636F7264696E67> Tj 0.48 Tc 1 0 0 1 70.32 451.44 Tm <746F20> Tj 1 0 0 1 82.08 451.68 Tm <666F726D756C613A20> Tj 1 0 0 1 120.24 452.16 Tm <256F20> Tj 1 0 0 1 131.28 452.40 Tm <696E6869626974696F6E20> Tj 1 0 0 1 173.76 454.80 Tm <3D20> Tj 1 0 0 1 181.44 450.96 Tm <5B20> Tj 1 0 0 1 185.04 453.60 Tm <28416F2E75752D412E2A2C222E2C292F34726F6F6E2920> Tj 1 0 0 1 270.48 452.16 Tm <5D2220> Tj 1 0 0 1 279.60 454.56 Tm <4920> Tj 1 0 0 1 283.92 454.56 Tm <303027> Tj 0.96 Tc /F3 11.0 Tf 1 0 0 1 71.52 422.16 Tm <48504C4320> Tj 1 0 0 1 102.24 422.64 Tm <616E616C7973697320> Tj 1 0 0 1 147.60 423.36 Tm <6F6620> Tj 1 0 0 1 160.80 423.60 Tm <666C61766F6E6F6C7320> Tj 1 0 0 1 211.20 424.32 Tm <616E6420> Tj 1 0 0 1 233.76 425.28 Tm <7068656E6F6C696320> Tj 1 0 0 1 281.04 425.28 Tm <6163696473> Tj 0.48 Tc /F3 9.0 Tf 1 0 0 1 71.28 407.76 Tm <466F7220> Tj 1 0 0 1 87.84 408.00 Tm <666C61766F6E6F6C20> Tj 1 0 0 1 124.56 408.48 Tm <616E6420> Tj 1 0 0 1 143.04 408.72 Tm <7068656E6F6C696320> Tj 1 0 0 1 181.92 409.44 Tm <6163696420> Tj 1 0 0 1 202.08 409.68 Tm <616E616C7673697320> Tj 1 0 0 1 237.36 410.16 Tm <627920> Tj 1 0 0 1 250.80 410.40 Tm <48504C4320> Tj 1 0 0 1 280.32 411.12 Tm <6D6574686F642C20> Tj 1 0 0 1 318.48 411.60 Tm <667275697420> Tj 1 0 0 1 339.60 411.84 Tm <6578747261637420> Tj 1 0 0 1 370.56 412.32 Tm <7765726520> Tj 1 0 0 1 392.88 412.56 Tm <707265706172656420> Tj 1 0 0 1 433.20 413.76 Tm <284869696B6B696E656E20> Tj 1 0 0 1 480.96 414.00 Tm <657420> Tj 1 0 0 1 491.76 414.24 Tm <616C2C20> Tj 1 0 0 1 505.44 414.48 Tm <3139393929> Tj 0.48 Tc 1 0 0 1 71.52 393.12 Tm <616E6420> Tj 1 0 0 1 90.00 393.36 Tm <616E616C7673656420> Tj 1 0 0 1 127.92 394.08 Tm <74686520> Tj 1 0 0 1 144.00 394.32 Tm <73616D6520> Tj 1 0 0 1 167.28 394.56 Tm <64617620> Tj 1 0 0 1 184.32 394.80 Tm <7768656E20> Tj 1 0 0 1 209.76 395.04 Tm <70726570617265642E20> Tj 1 0 0 1 250.56 396.00 Tm <4173636F7262696320> Tj 1 0 0 1 289.44 396.48 Tm <6163696420> Tj 1 0 0 1 309.84 396.96 Tm <28383020> Tj 1 0 0 1 326.64 396.96 Tm <6D672920> Tj 1 0 0 1 345.36 397.44 Tm <7276617320> Tj 1 0 0 1 363.84 397.68 Tm <646973736F6C76656420> Tj 1 0 0 1 404.88 398.40 Tm <696E20> Tj 1 0 0 1 415.92 398.40 Tm <64697374696C6C656420> Tj 1 0 0 1 451.20 399.12 Tm <776174657220> Tj 1 0 0 1 478.08 400.08 Tm <283520> Tj 1 0 0 1 489.36 399.60 Tm <6D6C2920> Tj 1 0 0 1 506.40 399.84 Tm <616E6420> Tj 1 0 0 1 524.88 400.08 Tm <35> Tj 0.48 Tc 1 0 0 1 71.76 378.24 Tm <6720> Tj 1 0 0 1 78.72 378.48 Tm <6F6620> Tj 1 0 0 1 89.28 378.72 Tm <686F6D6F67656E697A656420> Tj 1 0 0 1 148.08 379.68 Tm <667275697420> Tj 1 0 0 1 168.96 379.92 Tm <73616D706C652C20> Tj 1 0 0 1 203.04 380.40 Tm <323520> Tj 1 0 0 1 216.24 380.64 Tm <6D6C20> Tj 1 0 0 1 229.44 380.64 Tm <6F6620> Tj 1 0 0 1 240.24 380.88 Tm <6D657268616E6F6C20> Tj 1 0 0 1 282.48 381.60 Tm <616E6420> Tj 1 0 0 1 301.68 381.84 Tm <6C3020> Tj 1 0 0 1 313.92 382.08 Tm <6D6C20> Tj 1 0 0 1 327.12 382.32 Tm <6F6620> Tj 1 0 0 1 338.16 382.32 Tm <3620> Tj 1 0 0 1 345.84 382.56 Tm <4D20> Tj 1 0 0 1 357.60 382.80 Tm <48434920> Tj 1 0 0 1 377.52 383.04 Tm <7765726520> Tj 1 0 0 1 399.60 383.52 Tm <616464656420> Tj 1 0 0 1 427.44 383.76 Tm <746F20> Tj 1 0 0 1 438.48 384.00 Tm <6173636F7262696320> Tj 1 0 0 1 474.72 384.48 Tm <6163696420> Tj 1 0 0 1 494.16 384.96 Tm <736F6C7574696F6E27> Tj 0.48 Tc 1 0 0 1 72.00 363.84 Tm <576174657220> Tj 1 0 0 1 100.80 364.08 Tm <77617320> Tj 1 0 0 1 120.00 364.32 Tm <616464656420> Tj 1 0 0 1 149.04 364.80 Tm <746F20> Tj 1 0 0 1 161.28 365.04 Tm <7468697320> Tj 1 0 0 1 180.24 365.28 Tm <6D69787475726520> Tj 1 0 0 1 216.24 365.76 Tm <746F20> Tj 1 0 0 1 228.48 366.00 Tm <6F627461696E20> Tj 1 0 0 1 259.20 366.24 Tm <6120> Tj 1 0 0 1 267.36 366.48 Tm <66696E616C20> Tj 1 0 0 1 289.20 366.72 Tm <766F6C756D6520> Tj 1 0 0 1 324.00 367.44 Tm <6F6620> Tj 1 0 0 1 336.00 367.44 Tm <353020> Tj 1 0 0 1 350.40 367.92 Tm <6D6C20> Tj 1 0 0 1 365.04 368.16 Tm <616E6420> Tj 1 0 0 1 384.24 368.40 Tm <66696E616C20> Tj 1 0 0 1 406.56 368.64 Tm <636F6E63656E74726174696F6E20> Tj 1 0 0 1 468.24 369.60 Tm <6F6620> Tj 1 0 0 1 480.24 369.84 Tm <48434920> Tj 1 0 0 1 502.80 370.32 Tm <4920> Tj 1 0 0 1 509.76 370.32 Tm <3220> Tj 1 0 0 1 518.64 370.56 Tm <4D27> Tj 0.48 Tc 1 0 0 1 72.00 349.20 Tm <5468697320> Tj 1 0 0 1 94.32 349.44 Tm <736F6C7574696F6E20> Tj 1 0 0 1 130.80 349.92 Tm <77617320> Tj 1 0 0 1 149.76 350.40 Tm <7265666C7578656420> Tj 1 0 0 1 186.48 350.88 Tm <6F6E20> Tj 1 0 0 1 200.16 351.12 Tm <776174657220> Tj 1 0 0 1 226.56 351.36 Tm <6261746820> Tj 1 0 0 1 249.12 351.84 Tm <666F7220> Tj 1 0 0 1 265.20 352.08 Tm <6C3620> Tj 1 0 0 1 278.16 352.32 Tm <6820> Tj 1 0 0 1 287.04 352.32 Tm <617420> Tj 1 0 0 1 298.32 352.56 Tm <333520> Tj 1 0 0 1 312.72 354.72 Tm <224320> Tj 1 0 0 1 325.68 352.80 Tm <616E6420> Tj 1 0 0 1 344.40 353.28 Tm <7468616E20> Tj 1 0 0 1 367.20 353.76 Tm <66696C74657265642E20> Tj 1 0 0 1 402.00 354.24 Tm <4120> Tj 1 0 0 1 412.32 354.24 Tm <323020> Tj 1 0 0 1 426.48 354.48 Tm <6D6C20> Tj 1 0 0 1 440.64 354.72 Tm <706F7274696F6E20> Tj 1 0 0 1 474.96 355.20 Tm <6F6620> Tj 1 0 0 1 486.24 355.44 Tm <74686520> Tj 1 0 0 1 503.04 355.68 Tm <66696C7472617465> Tj 0.48 Tc 1 0 0 1 72.00 334.80 Tm <77617320> Tj 1 0 0 1 91.20 335.04 Tm <657661706F726174656420> Tj 1 0 0 1 140.64 335.76 Tm <746F20> Tj 1 0 0 1 152.88 336.00 Tm <6472766E65737320> Tj 1 0 0 1 188.40 336.48 Tm <6F6E20> Tj 1 0 0 1 202.56 336.72 Tm <6120> Tj 1 0 0 1 210.48 336.96 Tm <726F7461727620> Tj 1 0 0 1 239.52 337.20 Tm <657661706F7261746F7220> Tj 1 0 0 1 287.76 337.92 Tm <7573696E6720> Tj 1 0 0 1 312.96 338.40 Tm <6C766174657220> Tj 1 0 0 1 339.60 338.64 Tm <6261746820> Tj 1 0 0 1 362.40 339.12 Tm <616E6420> Tj 1 0 0 1 381.36 339.36 Tm <74656D706572617475726520> Tj 1 0 0 1 436.08 340.32 Tm <333527432720> Tj 1 0 0 1 462.72 340.80 Tm <54686520> Tj 1 0 0 1 482.88 341.04 Tm <7265736964756520> Tj 1 0 0 1 515.52 341.52 Tm <776173> Tj 0.48 Tc 1 0 0 1 72.72 319.92 Tm <646973736F6C76656420> Tj 1 0 0 1 114.00 320.64 Tm <696E20> Tj 1 0 0 1 125.04 320.88 Tm <3220> Tj 1 0 0 1 133.44 320.88 Tm <6D6C20> Tj 1 0 0 1 147.12 321.12 Tm <6F6620> Tj 1 0 0 1 158.40 321.36 Tm <6D657468616E6F6C20> Tj 1 0 0 1 201.12 321.84 Tm <616E6420> Tj 1 0 0 1 219.84 322.32 Tm <66696C746572656420> Tj 1 0 0 1 252.24 322.80 Tm <7468726F75676820> Tj 1 0 0 1 288.48 323.28 Tm <6120> Tj 1 0 0 1 295.92 323.28 Tm <302E27313520> Tj 1 0 0 1 317.28 324.00 Tm <706D20> Tj 1 0 0 1 334.32 324.00 Tm <737672696E676520> Tj 1 0 0 1 366.72 324.48 Tm <66696C74657220> Tj 1 0 0 1 390.00 325.44 Tm <285661726953657020> Tj 1 0 0 1 428.40 325.44 Tm <505446452C20> Tj 1 0 0 1 457.44 325.92 Tm <3027343520> Tj 1 0 0 1 478.80 326.64 Tm <70726D2C20> Tj 1 0 0 1 498.24 326.64 Tm <323520> Tj 1 0 0 1 512.16 326.88 Tm <6D6D2D> Tj 0.48 Tc 1 0 0 1 72.72 305.52 Tm <56617269616E2920> Tj 1 0 0 1 106.08 305.52 Tm <7072696F7220> Tj 1 0 0 1 128.88 306.24 Tm <746F20> Tj 1 0 0 1 140.16 306.48 Tm <696E6A656372696F6E20> Tj 1 0 0 1 179.28 306.96 Tm <696E746F20> Tj 1 0 0 1 198.72 307.20 Tm <74686520> Tj 1 0 0 1 214.80 307.44 Tm <48504C432E20> Tj 1 0 0 1 246.48 307.92 Tm <54686520> Tj 1 0 0 1 265.92 308.40 Tm <48504C4320> Tj 1 0 0 1 295.20 308.64 Tm <73767374656D20> Tj 1 0 0 1 326.40 309.12 Tm <656D706C6F76656420> Tj 1 0 0 1 369.84 309.84 Tm <636F6E73697374656420> Tj 1 0 0 1 411.12 310.56 Tm <6F6620> Tj 1 0 0 1 421.92 310.56 Tm <6120> Tj 1 0 0 1 428.64 310.80 Tm <56617269616E20> Tj 1 0 0 1 458.40 311.28 Tm <4C4320> Tj 1 0 0 1 473.76 311.52 Tm <73597374656D20> Tj 1 0 0 1 505.20 312.24 Tm <2855534129> Tj 0.48 Tc 1 0 0 1 73.44 290.40 Tm <657175697070656420> Tj 1 0 0 1 114.96 291.12 Tm <722C7669746820> Tj 1 0 0 1 137.76 291.36 Tm <6120> Tj 1 0 0 1 145.68 294.24 Tm <70726F5374617220> Tj 1 0 0 1 180.48 292.08 Tm <32333020> Tj 1 0 0 1 200.64 292.32 Tm <736F6C76656E7420> Tj 1 0 0 1 233.76 293.04 Tm <64656C697665727620> Tj 1 0 0 1 270.72 293.52 Tm <6D6F64756C652C20> Tj 1 0 0 1 308.40 294.24 Tm <50726F5374617220> Tj 1 0 0 1 343.44 294.48 Tm <33313020> Tj 1 0 0 1 362.88 294.96 Tm <572D56697320> Tj 1 0 0 1 396.24 295.44 Tm <4465746563746F722C20> Tj 1 0 0 1 438.00 296.16 Tm <616E6420> Tj 1 0 0 1 457.20 296.40 Tm <50726F5374617220> Tj 1 0 0 1 492.24 296.88 Tm <33333020> Tj 1 0 0 1 511.92 297.36 Tm <504441> Tj 0.48 Tc 1 0 0 1 73.68 276.00 Tm <4465746563746F722E20> Tj 1 0 0 1 114.96 276.48 Tm <466C61766F6E6F6C20> Tj 1 0 0 1 154.08 277.20 Tm <616E6420> Tj 1 0 0 1 172.32 277.20 Tm <7068656E6F6C696320> Tj 1 0 0 1 211.20 277.92 Tm <6163696420> Tj 1 0 0 1 231.12 278.16 Tm <73657061726174696F6E20> Tj 1 0 0 1 276.96 278.88 Tm <77617320> Tj 1 0 0 1 295.44 279.12 Tm <646F6E6520> Tj 1 0 0 1 319.20 279.60 Tm <696E20> Tj 1 0 0 1 330.24 279.60 Tm <6120> Tj 1 0 0 1 337.44 279.84 Tm <6F6D6E69737068657220> Tj 1 0 0 1 389.52 280.56 Tm <636C20> Tj 1 0 0 1 402.48 280.80 Tm <4220> Tj 1 0 0 1 410.40 281.04 Tm <636F6C756D6E20> Tj 1 0 0 1 445.20 282.00 Tm <2832353020> Tj 1 0 0 1 467.28 282.00 Tm <7820> Tj 1 0 0 1 474.72 282.00 Tm <34273620> Tj 1 0 0 1 491.04 282.24 Tm <6D6D20> Tj 1 0 0 1 510.48 282.48 Tm <696E6E6572> Tj 0.48 Tc 1 0 0 1 73.92 261.36 Tm <6469616D657465722C3520> Tj 1 0 0 1 121.92 262.32 Tm <70726D2C20> Tj 1 0 0 1 140.88 262.32 Tm <56617269616E2C20> Tj 1 0 0 1 172.80 262.80 Tm <55534129722C7669746820> Tj 1 0 0 1 219.60 263.52 Tm <6120> Tj 1 0 0 1 226.56 263.52 Tm <4368726F6D73657020> Tj 1 0 0 1 274.08 264.24 Tm <43494220> Tj 1 0 0 1 294.00 264.24 Tm <677561726420> Tj 1 0 0 1 320.16 264.96 Tm <636F6C756D6E20> Tj 1 0 0 1 354.48 265.92 Tm <286C20> Tj 1 0 0 1 365.28 265.68 Tm <636D7820> Tj 1 0 0 1 387.36 265.92 Tm <3320> Tj 1 0 0 1 394.80 266.16 Tm <6D6D2C20> Tj 1 0 0 1 415.92 266.64 Tm <56617269616E2720> Tj 1 0 0 1 447.84 266.88 Tm <555341292720> Tj 1 0 0 1 476.64 267.36 Tm <4D6F62696C6520> Tj 1 0 0 1 508.56 267.84 Tm <7068617365> Tj 0.48 Tc 1 0 0 1 73.68 246.96 Tm <4120> Tj 1 0 0 1 82.80 246.96 Tm <2A2C617320> Tj 1 0 0 1 101.04 247.20 Tm <302E3120> Tj 1 0 0 1 116.64 250.56 Tm <6F2F6F20> Tj 1 0 0 1 127.20 247.68 Tm <72766174657220> Tj 1 0 0 1 153.12 247.92 Tm <736F6C7574696F6E20> Tj 1 0 0 1 189.60 248.64 Tm <6F6620> Tj 1 0 0 1 200.16 248.40 Tm <70686F7370686F72696320> Tj 1 0 0 1 249.60 249.36 Tm <616369642C20> Tj 1 0 0 1 271.68 249.84 Tm <6D6F62696C6520> Tj 1 0 0 1 302.64 250.08 Tm <706861736520> Tj 1 0 0 1 329.04 250.56 Tm <4220> Tj 1 0 0 1 337.44 250.80 Tm 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C until analysis. For total anthoryanin, total pohphenol and antioxidant activity determination' threereplicates of fruit extracts were prepared and analvzed the same dav Fruit extracts for anthocvanin analvsis (l(altet al.,1999) \vere obtained bv grinding fruits (*5 g) in methanol (20 ml) acidified with HCI (0'l o/o' v/v) for2 min. The mlxture was stored at room temperature in the dark for 16 h and then filtered' Fruit extracts forpollphenolic analvsis (IGlt et al., 1999)were obtained bv grinding fruits (-5 S) in hot methanol (10 ml) for 2min. The solution was filtered, the residue was extracted again, tr,vo times, in the same wav and three extractswere combined. Fruit extracts for antioxidant activitv (Benvenuti et al, 2004) determination were obtained br'grinding fruits (-20 g) in methanol (20m1) acidified with HCI (0.lolo). After 60 min the solution was filtered'The residue was extracted again in the same wav. The extracts u'ere combined and the solution was diluted tovolume (50 ml) with methanol acidified with HCI (0' l%)'Total polvphenols were determined bY Folin-ciocalteau micro method (waterhouse, 2006) and expressed inmg of gallic acid equivalents (GAE) per kg of fruit. Total anthocvanins were estimated by a pH-differentialmethod (Giusti et al., 2001) and expressed in mg of cvaniclin-3-glucoside equivalents (CGE) per kg of fruitusingamolarexlinctronccrfficient (t:26900lmotr cm'r)andmolarweight (MW :149'2 gmolr)of o''anidin-3-glucoside. Data presented are mean + standard deviation (SD). Antioxidant actMty rvas determined usingthe 2,2-diphenvl-I-picrylhvdrazvl (DPPH) method (Benvenuti et al., 2004). Three or five dilutions of eachfruit extract were analvzed. Reaction solution rvas prepared by mlxing 50 pl of diluted fruit extract lvith 300pl of methanolic DPPH solution (ImM) and brought to 3 ml rvith methanol. The solution was kept in darkat room temperature for l5 minutes. The absorbance (A"".".) \l'as read against the prepared blank at 517 nm'The absorbance (A,,,oon) of DPPH blank solution (300 pl of lmM DPPH solution, 2'7 ml of methanol) wasmeasured daily. percent inhibition of DPPH radical r'vas caiculated for each dilution of fruit extract accordingto formula: %o inhibition = [ (Ao.uu-A.*,".,)/4roon) ]" I 00'HPLC analysis of flavonols and phenolic acidsFor flavonol and phenolic acid analvsis by HPLC method, fruit extract were prepared (Hiikkinen et al, 1999)and analvsed the same dav when prepared. Ascorbic acid (80 mg) rvas dissolved in distilled water (5 ml) and 5g of homogenized fruit sample, 25 ml of merhanol and l0 ml of 6 M HCI were added to ascorbic acid solution'Water was added to this mixture to obtain a final volume of 50 ml and final concentration of HCI I 2 M'This solution was refluxed on water bath for l6 h at 35 "C and than filtered. A 20 ml portion of the filtratewas evaporated to drvness on a rotarv evaporator using lvater bath and temperature 35'C' The residue wasdissolved in 2 ml of methanol and filtered through a 0.'15 pm svringe filter (VariSep PTFE, 0'45 prm, 25 mm-Varian) prior to injecrion into the HPLC. The HPLC svstem emploved consisted of a Varian LC sYstem (USA)equipped r,vith a proStar 230 solvent deliverv module, ProStar 310 W-Vis Detector, and ProStar 330 PDADetector. Flavonol and phenolic acid separation was done in a omnispher cl B column (250 x 4'6 mm innerdiameter,5 prm, Varian, USA)r,vith a Chromsep CIB guard column (l cmx 3 mm, Varian' USA)' Mobile phaseA *,as 0.1 o/o rvater solution of phosphoric acid, mobile phase B n'as 100 o/o HPLC grade methanol' The elutionconditions were as follows: 5-80 o/o B, 0-30 min; B0 o/o B 30-33 min; B0-5 o/o B, 33-35 min; with florv rate 0'Bml min'r. Operating conditions were as follows: column temperature 20'C; iniection volume I0 pi, wavelengthrange from 190-600 nm (detection r,vaveiength for p-hvdroxvbenzoic and ellagic acid was 260; for p-coumaric,caffeic and ferulic acid 320 nm; for flavonols 360 nm). Identification and peak assignment of flavonols andphenolic acids rvas based on comparison of their retention times and spectral data (I90-600 nm) rvith those ofauthentic standards. Identifiecl phenolic compounds were ex?ressed as o/o of total peak area.Results and discussionAnthocYanins (Table l) rvere found in the highest concentrations in elderberrv (6544 mg Lg'),blueberrl'(4979 mgkgr), and black currant (2809 mg kg'), whereas their concentration in red currant and sour cherrvwere considerablv lorver (257ngkgr,475 mg kgr, respectivelv). Polyphenols (Table l) rvere found in thehighest concentrations in elderberrr', blueberrv ancl black currant (8439 mg kgr, 5969 mg kg" a626 mg kg 634 4i, ililVAl${l I 2" l"{[fiLlhlAt*l]l'll $ll'1f*;lj A*A*ru*'UA endstream endobj 17 0 obj 4721 endobj 18 0 obj << /Length 27 >> stream % CANON_PFINF_TYPE0_TEXTON endstream endobj 19 0 obj << /Length 45 >> stream q 597.12 0 0 835.20 0.00 0.00 cm /Obj13 Do Q endstream endobj 20 0 obj << /Type /Page /MediaBox [ 0 0 597.12 835.20 ] /Parent 11 0 R /Resources << /Font << /F3 5 0 R >> /XObject << /Obj13 13 0 R >> /Subtype 16 0 R /ProcSet [ /PDF /Text /ImageB /ImageC /ImageI ] >> /Contents [ 18 0 R 19 0 R 14 0 R ] >> endobj 21 0 obj << /Type /XObject /Subtype /Image /Width 2488 /Height 3480 /BitsPerComponent 1 /ColorSpace /DeviceGray /Filter /CCITTFaxDecode /DecodeParms << /K -1 /Columns 2488 >> /Length 60608 >> stream ,@2fG.t]菗EqE:A$A$A$dqA0A& """pGɎq98L'8HIB":(t c莬Dsq98sq8A0 Lv&I I N8q@E"98sq98 )A H$A A B#rܧ)us qH$ QNL& a4IDtI!@Jr).q98tA H$!A0Bi""## ;9N&A^q:Gq:H$ I$ l& DDGxA CG8㤑I$:I$A IXA0L&XB"8!, ELq98t8$H$A+  a DDDGDA98r;8H L)8㤒I$I $bL& Gsq98 L&G#I I$I J BA#sq918A2> :I$I$G$DR[ a0DDGȣ98pa2>Ga0"I$B"""sB"""qɎq8"?sq8A0La0S:I$""""?Nq91sqI%sq8A0Ad|&A0  Ј#B g㤑NA Ksq a0L a0CH$I B?! 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1 449.52 760.80 Tm <283131353020> Tj 1 0 0 1 478.56 760.08 Tm <6D67> Tj 0.72 Tc 1 0 0 1 32.16 752.64 Tm <6C3C67742C3231373220> Tj 1 0 0 1 79.68 751.92 Tm <6D6720> Tj 1 0 0 1 96.48 751.68 Tm <6B67722C20> Tj 1 0 0 1 117.84 751.44 Tm <726573706563746976656C76292E20> Tj 1 0 0 1 176.40 750.48 Tm <4163636F7264696E67746F20> Tj 1 0 0 1 236.40 749.52 Tm <6461746120> Tj 1 0 0 1 258.96 749.04 Tm <70726573636E74636420> Tj 1 0 0 1 303.60 748.32 Tm <627620> Tj 1 0 0 1 317.76 748.08 Tm <6F7468657220> Tj 1 0 0 1 344.16 747.84 Tm <617574686F72732C20> Tj 1 0 0 1 382.56 747.12 Tm <656C64657262657272762C20> Tj 1 0 0 1 431.28 746.40 Tm <626C7565626572727620> Tj 1 0 0 1 475.44 745.68 Tm <616E64> Tj 0.48 Tc 1 0 0 1 31.92 738.24 Tm <626C61636B20> Tj 1 0 0 1 57.12 737.76 Tm <63757272616E7420> Tj 1 0 0 1 91.20 737.28 Tm <636F6E7461696E65636C20> Tj 1 0 0 1 135.84 736.80 Tm <68696768657220> Tj 1 0 0 1 165.60 736.08 Tm <636F6E63656E74726174696F6E7320> Tj 1 0 0 1 230.88 735.12 Tm <6F6620> Tj 1 0 0 1 242.40 734.88 Tm <706F6C797068656E3C6C6C7320> Tj 1 0 0 1 296.64 733.92 Tm <616E6420> Tj 1 0 0 1 315.60 733.68 Tm <616E74686F6376616E6972727320> Tj 1 0 0 1 375.36 732.72 Tm <7468616E20> Tj 1 0 0 1 397.68 732.48 Tm <66727569747320> Tj 1 0 0 1 423.36 732.24 Tm <6C696B6520> Tj 1 0 0 1 441.12 732.00 Tm <72656420> Tj 1 0 0 1 457.68 731.52 Tm <63757272616E742C> Tj 0.48 Tc 1 0 0 1 31.68 723.60 Tm <626C61636B626572727620> Tj 1 0 0 1 78.96 722.88 Tm <616E6420> Tj 1 0 0 1 97.20 722.64 Tm <72617370626572727620> Tj 1 0 0 1 139.92 722.40 Tm <2842656E76656E75746920> Tj 1 0 0 1 188.40 721.20 Tm <657420> Tj 1 0 0 1 198.96 720.96 Tm <61692E2C20> Tj 1 0 0 1 213.60 720.72 Tm <32303027313B20> Tj 1 0 0 1 240.72 720.24 Tm <49476C7420> Tj 1 0 0 1 260.88 720.00 Tm <657420> Tj 1 0 0 1 271.20 719.76 Tm <616C2C20> Tj 1 0 0 1 284.64 719.76 Tm <313939392920> Tj 1 0 0 1 311.04 719.28 Tm <72766869636820> Tj 1 0 0 1 339.12 718.80 Tm <616772656520> Tj 1 0 0 1 362.64 718.32 Tm <7769746820> Tj 1 0 0 1 384.24 718.08 Tm <6F757220> Tj 1 0 0 1 400.80 717.84 Tm <726573756C74732E20> Tj 1 0 0 1 432.00 717.12 Tm <416E7468366376616E696E73> Tj 0.96 Tc 1 0 0 1 31.44 708.96 Tm <7276657265746865707265646F6D696E616E74706F6C767068656E6F6C6963636F6D706F6E656E7473696E626C756562657272762838332572292C656C646572626572727620> Tj 1 0 0 1 376.32 704.16 Tm <2837366F68296F72626C61636B63757272616E74283631> Tj 0.48 Tc 1 0 0 1 31.44 694.08 Tm <376F2920> Tj 1 0 0 1 45.60 693.60 Tm <72277668657265617320> Tj 1 0 0 1 82.08 693.12 Tm <74686520> Tj 1 0 0 1 98.40 692.88 Tm <706F7274696F6E20> Tj 1 0 0 1 132.24 692.40 Tm <6F6620> Tj 1 0 0 1 143.52 692.16 Tm <616E74686F6376616E696E7320> Tj 1 0 0 1 202.80 691.20 Tm <696E20> Tj 1 0 0 1 213.84 691.20 Tm <72656420> Tj 1 0 0 1 229.68 690.72 Tm <63757272616E7420> Tj 1 0 0 1 263.76 690.72 Tm <28323220> Tj 1 0 0 1 280.80 690.00 Tm <566F2920> Tj 1 0 0 1 295.44 689.52 Tm <616E6420> Tj 1 0 0 1 314.16 689.28 Tm <736F757220> Tj 1 0 0 1 334.56 689.04 Tm <636865726E6E2C20> Tj 1 0 0 1 365.04 689.04 Tm <283139256F2920> Tj 1 0 0 1 393.60 688.32 Tm <722C76617320> Tj 1 0 0 1 412.08 687.84 Tm <636F277369636C657261626C7620> Tj 1 0 0 1 467.52 687.12 Tm <6C6F776572> Tj 0.72 Tc 1 0 0 1 31.68 681.12 Tm <285461626C6320> Tj 1 0 0 1 61.44 678.96 Tm <4920> Tj 1 0 0 1 65.76 677.04 Tm <29> Tj 0.72 Tc 1 0 0 1 30.72 652.32 Tm <5461626C6520> Tj 1 0 0 1 57.36 651.84 Tm <6C2E20> Tj 1 0 0 1 74.88 651.60 Tm <436F6E63656E74726174696F6E7320> Tj 1 0 0 1 143.76 650.40 Tm <6F6620> Tj 1 0 0 1 155.04 650.16 Tm <746F743A726C20> Tj 1 0 0 1 177.84 649.92 Tm <616E72686F6376616E696E7320> Tj 1 0 0 1 238.56 649.20 Tm <2854412920> Tj 1 0 0 1 261.84 648.72 Tm <286D6720> Tj 1 0 0 1 280.80 648.24 Tm <4347452F3C67292C20> Tj 1 0 0 1 323.52 647.52 Tm <746F74616C20> Tj 1 0 0 1 346.32 647.04 Tm <706F6C767068656E6F6C7320> Tj 1 0 0 1 402.00 646.80 Tm <285449722920> Tj 1 0 0 1 425.04 646.32 Tm <286D67> Tj 0.72 Tc 1 0 0 1 74.64 638.40 Tm <4741452C343C2E677420> Tj 1 0 0 1 114.24 637.92 Tm <616E6420> Tj 1 0 0 1 133.20 637.68 Tm <5441222F547C2920> Tj 1 0 0 1 164.64 637.20 Tm <726174696F> Tj 0.72 Tc /F3 10.0 Tf 1 0 0 1 33.84 617.52 Tm <42657272696573> Tj 0.48 Tc /F3 9.0 Tf 1 0 0 1 144.48 622.56 Tm <546F74616C20> Tj 1 0 0 1 169.20 622.08 Tm <616E74686F6376616E696E73> Tj 0.72 Tc /F3 10.0 Tf 1 0 0 1 289.20 619.92 Tm <546F74616C20> Tj 1 0 0 1 313.92 619.44 Tm <706F6C767068656E6F6C73> Tj 0.72 Tc 1 0 0 1 33.12 593.52 Tm <426C75656265727276> Tj 0.72 Tc 1 0 0 1 32.88 580.56 Tm <456C6465726265727276> Tj 0.72 Tc 1 0 0 1 32.64 567.60 Tm <426C61636B20> Tj 1 0 0 1 58.80 567.12 Tm <63757272616E74> Tj 0.48 Tc 1 0 0 1 32.40 554.40 Tm <52656420> Tj 1 0 0 1 51.84 553.92 Tm <63757272616E74> Tj 0.72 Tc 1 0 0 1 32.64 540.96 Tm <536F757220> Tj 1 0 0 1 55.20 540.48 Tm <636865727276> Tj 0.96 Tc /F3 11.0 Tf 1 0 0 1 127.68 592.32 Tm <313937382E3932> Tj 0.96 Tc 1 0 0 1 127.44 579.12 Tm <363534342E3031> Tj 1.20 Tc 1 0 0 1 126.24 566.16 Tm <323830392E3333> Tj 1.50 Tc 1 0 0 1 128.88 552.96 Tm <3235372E3431> Tj 1.20 Tc 1 0 0 1 128.64 539.52 Tm <3437312E3731> Tj 0.00 Tc /F3 4.0 Tf 1 0 0 1 320.16 592.56 Tm <2D66> Tj 0.00 Tc 1 0 0 1 319.92 579.60 Tm <2D6C2D> Tj 0.00 Tc 1 0 0 1 319.92 566.64 Tm <2D66> Tj 0.00 Tc /F3 8.0 Tf 1 0 0 1 319.68 551.52 Tm <2B> Tj 0.00 Tc /F3 5.0 Tf 1 0 0 1 319.44 540.00 Tm <2D742D> Tj 1.20 Tc /F3 11.0 Tf 1 0 0 1 181.20 594.72 Tm <2D20> Tj 1 0 0 1 211.20 590.64 Tm <3738> Tj 1.50 Tc /F3 9.0 Tf 1 0 0 1 181.20 580.08 Tm <2B3535> Tj 0.48 Tc 1 0 0 1 180.96 568.80 Tm <2D6620> Tj 1 0 0 1 210.96 564.72 Tm <3736> Tj 0.48 Tc 1 0 0 1 180.72 555.60 Tm <2D6620> Tj 1 0 0 1 210.24 551.52 Tm <3230> Tj 1.50 Tc 1 0 0 1 180.72 540.72 Tm <2B36> Tj 0.96 Tc /F3 10.0 Tf 1 0 0 1 266.64 589.92 Tm <353936382E3720> Tj 1 0 0 1 296.40 589.44 Tm <35> Tj 1.20 Tc 1 0 0 1 265.68 576.96 Tm <383433392E3334> Tj 0.96 Tc 1 0 0 1 266.16 564.00 Tm <343632352E3931> Tj 1.20 Tc 1 0 0 1 266.16 550.56 Tm <4920> Tj 1 0 0 1 271.68 550.56 Tm <6C2C7B672E6742> Tj 1.44 Tc 1 0 0 1 265.20 537.12 Tm <32343720> Tj 1 0 0 1 283.20 537.12 Tm <6C2E3934> Tj 0.48 Tc /F3 9.0 Tf 1 0 0 1 315.12 606.72 Tm <6E72672F6C3C6729> Tj 0.00 Tc /F3 11.0 Tf 1 0 0 1 410.64 611.76 Tm <5441494950> Tj 1.20 Tc 1 0 0 1 414.72 587.52 Tm <302E3833> Tj 1.44 Tc 1 0 0 1 414.72 574.56 Tm <302E3736> Tj 1.50 Tc 1 0 0 1 414.48 561.36 Tm <302E3631> Tj 1.20 Tc 1 0 0 1 414.24 548.16 Tm <302E3232> Tj 1.50 Tc 1 0 0 1 414.24 534.72 Tm <302E7239> Tj 1.50 Tc 1 0 0 1 346.32 588.72 Tm <327449> Tj 1.50 Tc /F3 7.0 Tf 1 0 0 1 349.20 577.68 Tm <376C> Tj 1.50 Tc /F3 11.0 Tf 1 0 0 1 345.84 562.56 Tm <337435> Tj 1.50 Tc 1 0 0 1 348.48 549.12 Tm <3654> Tj 1.50 Tc 1 0 0 1 346.32 535.92 Tm <313338> Tj 0.48 Tc /F3 9.0 Tf 1 0 0 1 28.56 508.56 Tm <416C6C20> Tj 1 0 0 1 44.64 508.32 Tm <696E7665737469676174656420> Tj 1 0 0 1 98.88 507.60 Tm <667275697420> Tj 1 0 0 1 121.44 507.12 Tm <657874726163747320> Tj 1 0 0 1 157.68 506.40 Tm <65786869626974656420> Tj 1 0 0 1 200.64 505.68 Tm <706F74656E7420> Tj 1 0 0 1 232.32 505.44 Tm <7261646963616C20> Tj 1 0 0 1 264.48 504.72 Tm <73636176656E67696E6720> Tj 1 0 0 1 313.44 504.00 Tm <616374697669747620> Tj 1 0 0 1 348.96 504.00 Tm <2846696775726520> Tj 1 0 0 1 383.04 503.04 Tm <6C292E20> Tj 1 0 0 1 397.44 502.80 Tm <54686520> Tj 1 0 0 1 418.56 502.32 Tm <7374726F6E6765737420> Tj 1 0 0 1 459.84 501.84 Tm <7261646963616C> Tj 0.48 Tc 1 0 0 1 29.04 493.92 Tm <73636176656E67696E6720> Tj 1 0 0 1 77.28 493.20 Tm <616374697669747620> Tj 1 0 0 1 112.08 492.72 Tm <73686F7276656420> Tj 1 0 0 1 146.88 492.24 Tm <626C75656265727272272C20> Tj 1 0 0 1 192.24 491.28 Tm <656C6465726265727272272720> Tj 1 0 0 1 239.04 490.56 Tm <616E6420> Tj 1 0 0 1 258.24 490.32 Tm <626C61636C3C20> Tj 1 0 0 1 283.92 489.84 Tm <63757272616E742C20> Tj 1 0 0 1 320.64 489.36 Tm <722C722E68696C6520> Tj 1 0 0 1 346.80 488.88 Tm <6163746976697469657320> Tj 1 0 0 1 387.60 488.40 Tm <6F6620> Tj 1 0 0 1 399.36 488.16 Tm <72656420> Tj 1 0 0 1 416.16 487.92 Tm <63757272616E7420> Tj 1 0 0 1 450.48 487.20 Tm <616E6420> Tj 1 0 0 1 469.92 486.96 Tm <736F7572> Tj 0.48 Tc 1 0 0 1 28.56 479.28 Tm <63686572727620> Tj 1 0 0 1 57.84 478.80 Tm <722C7665726520> Tj 1 0 0 1 80.40 478.56 Tm <636F6E736964657261626C7620> Tj 1 0 0 1 135.84 477.84 Tm <6C6F6C722C65722E> Tj 0.72 Tc 1 0 0 1 76.08 354.24 Tm <3020> Tj 1 0 0 1 117.36 353.52 Tm <302C30303120> Tj 1 0 0 1 166.08 352.80 Tm <302C30303220> Tj 1 0 0 1 214.80 352.08 Tm <302C30303320> Tj 1 0 0 1 263.52 351.12 Tm <302C303034> Tj 0.24 Tc 1 0 0 1 137.28 340.56 Tm <436F6E63656E74726174696F6E20> Tj 1 0 0 1 190.56 340.32 Tm <28672F6D6C29> Tj 0.24 Tc 1 0 0 1 41.04 329.76 Tm <2D2A2D656C646572626572727920> Tj 1 0 0 1 125.52 328.56 Tm <2D742D20> Tj 1 0 0 1 158.64 326.64 Tm <626C7565626572727920> Tj 1 0 0 1 209.52 327.12 Tm <5F20> Tj 1 0 0 1 218.64 327.12 Tm <2D412D20> Tj 1 0 0 1 236.64 326.64 Tm <2D20> Tj 1 0 0 1 243.12 325.20 Tm <626C61636B637572723A6D72> Tj 0.24 Tc 1 0 0 1 41.52 315.12 Tm <7120> Tj 1 0 0 1 66.00 314.88 Tm <2D20> Tj 1 0 0 1 74.64 312.96 Tm <72656463757272613A727420> Tj 1 0 0 1 124.32 313.68 Tm <2D7B6C2D736F75726368656E76> Tj 0.48 Tc 1 0 0 1 26.64 274.32 Tm <4669717272726520> Tj 1 0 0 1 55.92 273.84 Tm <6C2E20> Tj 1 0 0 1 65.28 273.60 Tm <5261646963616C20> Tj 1 0 0 1 99.12 272.88 Tm <73636176656E67696E6720> Tj 1 0 0 1 146.88 272.16 Tm <6163746976697469657320> Tj 1 0 0 1 186.72 271.44 Tm <6F6620> Tj 1 0 0 1 198.00 271.44 Tm <667275697420> Tj 1 0 0 1 219.12 270.96 Tm <65787472616374732E> Tj 0.48 Tc 1 0 0 1 26.16 245.28 Tm <6C2763742D63656E7420> Tj 1 0 0 1 60.72 244.56 Tm <646973747269627574696F6E20> Tj 1 0 0 1 114.72 243.84 Tm <6F6620> Tj 1 0 0 1 127.68 243.60 Tm <696E646976696475616C20> Tj 1 0 0 1 174.48 242.64 Tm <666C61766F6E6F6C7320> Tj 1 0 0 1 216.72 241.92 Tm <616E6420> Tj 1 0 0 1 236.88 241.44 Tm <7068656E6F6C696320> Tj 1 0 0 1 277.20 240.96 Tm <616369647320> Tj 1 0 0 1 302.64 240.48 Tm <696E20> Tj 1 0 0 1 315.60 240.24 Tm <66727569747320> Tj 1 0 0 1 342.24 239.76 Tm <61726520> Tj 1 0 0 1 359.28 239.52 Tm <73686F722C722E6E20> Tj 1 0 0 1 390.72 239.04 Tm <696E20> Tj 1 0 0 1 403.44 238.80 Tm <6C61626C6520> Tj 1 0 0 1 430.32 238.32 Tm <322E20> Tj 1 0 0 1 443.28 238.08 Tm <426C75656265727276> Tj 0.72 Tc 1 0 0 1 25.68 230.16 Tm <27722972727461696E656420> Tj 1 0 0 1 70.08 229.44 Tm <666C61766F6E6F6C7320> Tj 1 0 0 1 110.64 228.96 Tm <6D767269636574696E2C20> Tj 1 0 0 1 156.48 228.00 Tm <71756572636574696E20> Tj 1 0 0 1 198.96 227.28 Tm <616E6420> Tj 1 0 0 1 217.92 227.04 Tm <6B61656D706665726F6C2C20> Tj 1 0 0 1 270.48 226.08 Tm <6F6620> Tj 1 0 0 1 281.52 225.84 Tm <776869636820> Tj 1 0 0 1 310.08 225.36 Tm <74686520> Tj 1 0 0 1 327.12 225.36 Tm <6D6F737420> Tj 1 0 0 1 350.64 224.88 Tm <6162756E64616E7477617320> Tj 1 0 0 1 412.80 223.68 Tm <717565726365746920> Tj 1 0 0 1 446.40 223.44 Tm <6E20> Tj 1 0 0 1 455.52 223.44 Tm <283532566F292E> Tj 0.72 Tc 1 0 0 1 25.92 215.52 Tm <6C2768722772726F6C696320> Tj 1 0 0 1 65.28 214.80 Tm <616369647320> Tj 1 0 0 1 90.24 214.56 Tm <666F756E6420> Tj 1 0 0 1 119.04 214.08 Tm <696E20> Tj 1 0 0 1 131.04 213.60 Tm <626C7565626572727620> Tj 1 0 0 1 175.20 213.12 Tm <7765726520> Tj 1 0 0 1 198.72 212.40 Tm <702D636F756D6172696320> Tj 1 0 0 1 250.08 212.16 Tm <28313825292C20> Tj 1 0 0 1 282.48 211.20 Tm <6361666665696320> Tj 1 0 0 1 313.92 211.20 Tm <286C326F2F6F2920> Tj 1 0 0 1 346.08 210.24 Tm <616E6466656E726C696320> Tj 1 0 0 1 393.84 209.52 Tm <6163696420> Tj 1 0 0 1 415.44 209.52 Tm <283225292E20> Tj 1 0 0 1 442.08 208.80 Tm <54686520> Tj 1 0 0 1 462.72 208.32 Tm <6D61696E> Tj 0.48 Tc 1 0 0 1 25.20 198.24 Tm <6C726C726572723C726C696320> Tj 1 0 0 1 63.36 200.40 Tm <636F6D706F756E6420> Tj 1 0 0 1 111.60 199.68 Tm <696E20> Tj 1 0 0 1 122.40 199.44 Tm <656C646520> Tj 1 0 0 1 139.68 199.20 Tm <72626572727620> Tj 1 0 0 1 168.00 198.72 Tm <77617320> Tj 1 0 0 1 186.48 198.00 Tm <71756572636574696E20> Tj 1 0 0 1 228.96 198.24 Tm <283820> Tj 1 0 0 1 238.80 197.52 Tm <4920> Tj 1 0 0 1 243.12 197.28 Tm <25292C20> Tj 1 0 0 1 260.64 197.28 Tm <666F6C6C6F77656420> Tj 1 0 0 1 298.80 196.32 Tm <627620> Tj 1 0 0 1 312.00 196.08 Tm <6361666665696320> Tj 1 0 0 1 341.52 195.84 Tm <6163696420> Tj 1 0 0 1 361.92 195.84 Tm <2820> Tj 1 0 0 1 366.48 195.36 Tm <4920> Tj 1 0 0 1 370.56 195.36 Tm <3025292C20> Tj 1 0 0 1 393.12 194.88 Tm <702D636F756D6172696320> Tj 1 0 0 1 445.68 194.16 Tm <6163696420> Tj 1 0 0 1 463.44 194.16 Tm <28376F2F6F29> Tj 0.72 Tc 1 0 0 1 24.96 186.48 Tm <617272636920> Tj 1 0 0 1 43.92 186.24 Tm <6B61656E72706665726F6C20> Tj 1 0 0 1 94.56 185.76 Tm <286C376F292E20> Tj 1 0 0 1 120.96 185.04 Tm <496E20> Tj 1 0 0 1 133.44 184.80 Tm <626C61636B20> Tj 1 0 0 1 158.88 184.32 Tm <63757272616E742C20> Tj 1 0 0 1 195.60 183.84 Tm <74686520> Tj 1 0 0 1 212.64 183.36 Tm <6D61696F7220> Tj 1 0 0 1 240.00 182.88 Tm <7068656E6F6C696320> Tj 1 0 0 1 279.36 182.16 Tm <636F6D706F756E6420> Tj 1 0 0 1 327.36 181.44 Tm <6C76617320> Tj 1 0 0 1 346.56 181.20 Tm <6D767269636574696E20> Tj 1 0 0 1 390.72 180.96 Tm <283338376F292C20> Tj 1 0 0 1 422.64 180.24 Tm <666F696C6F752C656420> Tj 1 0 0 1 461.52 179.52 Tm <627920> Tj 1 0 0 1 475.20 179.04 Tm <702D> Tj 0.48 Tc 1 0 0 1 24.48 171.84 Tm <636F756D6172696320> Tj 1 0 0 1 65.04 171.36 Tm <6163696420> Tj 1 0 0 1 84.72 171.84 Tm <283220> Tj 1 0 0 1 94.80 170.88 Tm <4920> Tj 1 0 0 1 98.88 173.76 Tm <6F2F6F292C20> Tj 1 0 0 1 115.44 170.40 Tm <71756572636574696E20> Tj 1 0 0 1 157.20 170.40 Tm <286C20> Tj 1 0 0 1 166.32 169.68 Tm <36306C6F292C20> Tj 1 0 0 1 187.92 169.20 Tm <636166662765696320> Tj 1 0 0 1 216.96 168.96 Tm <616369637420> Tj 1 0 0 1 236.40 169.20 Tm <28312C7B256F292E20> Tj 1 0 0 1 267.12 168.00 Tm <54686520> Tj 1 0 0 1 285.84 167.76 Tm <6C6576656C7320> Tj 1 0 0 1 310.80 167.28 Tm <6F6620> Tj 1 0 0 1 321.12 167.04 Tm <656C6C6167696320> Tj 1 0 0 1 349.20 166.56 Tm <616369636C2C20> Tj 1 0 0 1 371.28 166.56 Tm <666572756C696320> Tj 1 0 0 1 399.60 165.84 Tm <6163696420> Tj 1 0 0 1 418.80 165.60 Tm <616E6420> Tj 1 0 0 1 436.56 165.12 Tm <6B61656D706665726F6C> Tj 0.48 Tc 1 0 0 1 24.00 157.44 Tm <727665726520> Tj 1 0 0 1 46.08 156.96 Tm <6C6F72762720> Tj 1 0 0 1 65.28 156.48 Tm <52656420> 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<3130302E3030> Tj 1.50 Tc 1 0 0 1 447.36 466.32 Tm <312E723720> Tj 1 0 0 1 490.80 466.08 Tm <3130302E3030> Tj 1.20 Tc 1 0 0 1 446.16 452.88 Tm <322E323820> Tj 1 0 0 1 490.08 452.64 Tm <3130302E3030> Tj 1.20 Tc 1 0 0 1 446.16 439.68 Tm <302E373620> Tj 1 0 0 1 490.32 439.68 Tm <7230302E3030> Tj 1.20 Tc 1 0 0 1 447.36 426.96 Tm <6C2E383320> Tj 1 0 0 1 490.08 426.48 Tm <3130302E3030> Tj 1.20 Tc /F3 11.0 Tf 1 0 0 1 138.96 441.60 Tm <36332E3731> Tj 0.72 Tc /F3 12.0 Tf 1 0 0 1 68.64 381.12 Tm <5265666572656E636573> Tj 0.48 Tc /F3 9.0 Tf 1 0 0 1 68.16 366.48 Tm <4265617474696520> Tj 1 0 0 1 101.76 364.56 Tm <312E2C20> Tj 1 0 0 1 114.72 366.00 Tm <43726F7A74657220> Tj 1 0 0 1 148.56 366.00 Tm <412E2C20> Tj 1 0 0 1 165.36 365.76 Tm <44757468696520> Tj 1 0 0 1 198.96 365.52 Tm <472E20> Tj 1 0 0 1 213.60 366.00 Tm <2832303035292E20> Tj 1 0 0 1 249.12 365.28 Tm <506F74656E7469616C20> Tj 1 0 0 1 290.64 365.04 Tm <6865616C746820> Tj 1 0 0 1 320.88 364.80 Tm <62656E656669747320> Tj 1 0 0 1 358.08 364.56 Tm <6F6620> Tj 1 0 0 1 370.32 364.56 Tm <626572726965732E20> Tj 1 0 0 1 405.12 364.32 Tm <43757272656E7420> Tj 1 0 0 1 442.08 364.32 Tm <4E7574726974696F6E20> Tj 1 0 0 1 486.48 363.84 Tm <616E6420> Tj 1 0 0 1 506.16 363.84 Tm <466F6F64> Tj 1.44 Tc 1 0 0 1 82.32 351.84 Tm <536369656E636520> Tj 1 0 0 1 116.88 352.56 Tm <286C293A37312D3836> Tj 0.72 Tc 1 0 0 1 68.16 337.68 Tm <42656E76656E7574692C20> Tj 1 0 0 1 118.08 337.20 Tm <532E2C20> Tj 1 0 0 1 132.72 337.20 Tm <50656C6C6174692C20> Tj 1 0 0 1 165.36 336.96 Tm <462E2C20> Tj 1 0 0 1 178.32 336.96 Tm <4D656C65676172692C20> Tj 1 0 0 1 222.00 336.72 Tm <4D2E2C20> Tj 1 0 0 1 240.72 336.48 Tm <42657274656C6C692C20> Tj 1 0 0 1 278.16 336.24 Tm <442E20> Tj 1 0 0 1 293.04 336.48 Tm <2832303034292E20> Tj 1 0 0 1 329.04 336.00 Tm <506F6C767068656E6F6C732C20> Tj 1 0 0 1 386.40 335.52 Tm <616E74686F6376616E696E732C20> Tj 1 0 0 1 449.52 335.28 Tm <6173636F7262696320> Tj 1 0 0 1 487.44 335.04 Tm <616369642C20> Tj 1 0 0 1 511.20 334.80 Tm <61727264> Tj 0.48 Tc 1 0 0 1 82.08 322.80 Tm <7261646963616C20> Tj 1 0 0 1 112.56 322.56 Tm <73636176656E67696E6720> Tj 1 0 0 1 160.56 322.32 Tm <616374697669747620> Tj 1 0 0 1 194.16 322.08 Tm <6F6620> Tj 1 0 0 1 205.68 321.84 Tm <52756275732C20> Tj 1 0 0 1 237.12 321.60 Tm <52696265732C20> Tj 1 0 0 1 265.44 321.60 Tm <616E6420> Tj 1 0 0 1 283.44 321.36 Tm <41726F6E69612E20> Tj 1 0 0 1 317.52 319.44 Tm <6C6F75726E616C20> Tj 1 0 0 1 350.88 320.88 Tm <6F6620> Tj 1 0 0 1 362.40 321.12 Tm <466F6F6420> Tj 1 0 0 1 386.40 320.64 Tm <536369656E636520> Tj 1 0 0 1 420.72 321.12 Tm <283639293A20> Tj 1 0 0 1 445.44 320.64 Tm <4920> Tj 1 0 0 1 450.96 320.40 Tm <36342D313639> Tj 0.48 Tc 1 0 0 1 67.92 308.16 Tm <4769757374692C20> Tj 1 0 0 1 100.80 307.92 Tm <4D2E4D2E2C20> Tj 1 0 0 1 132.00 307.68 Tm <57726F6C737461642C20> Tj 1 0 0 1 177.36 307.44 Tm <522E382E2C20> Tj 1 0 0 1 203.04 307.68 Tm <2832303031292E20> Tj 1 0 0 1 238.32 306.96 Tm <416E74686F6376616E696E732E20> Tj 1 0 0 1 304.32 306.48 Tm <436861726163746572697A6174696F6E20> Tj 1 0 0 1 379.20 306.24 Tm <616E6420> Tj 1 0 0 1 399.36 306.00 Tm <6D6561737572656D656E7420> Tj 1 0 0 1 459.84 305.76 Tm <727669746820> Tj 1 0 0 1 483.12 305.28 Tm <55562D76697369626C65> Tj 0.48 Tc 1 0 0 1 82.08 293.28 Tm <7370656374726F73636F70792E20> Tj 1 0 0 1 141.12 293.04 Tm <4972723A20> Tj 1 0 0 1 156.72 292.80 Tm <43757272656E7420> Tj 1 0 0 1 193.92 292.56 Tm <70726F746F636F6C7320> Tj 1 0 0 1 236.88 292.32 Tm <696E20> Tj 1 0 0 1 249.36 292.32 Tm <666F6F6420> Tj 1 0 0 1 272.64 292.08 Tm <616E616C722E746963616C20> Tj 1 0 0 1 316.80 291.60 Tm <6368656D697374727620> Tj 1 0 0 1 363.36 291.84 Tm <28522E452E20> Tj 1 0 0 1 388.56 291.36 Tm <57726F6C7374616420> Tj 1 0 0 1 431.04 291.12 Tm <6564292C20> Tj 1 0 0 1 450.96 290.88 Tm <57696C65762C20> Tj 1 0 0 1 481.92 290.88 Tm <4E65727620> Tj 1 0 0 1 504.96 290.64 Tm <596F726B2C> Tj 1.50 Tc 1 0 0 1 81.84 278.88 Tm <466C2E322E3120> Tj 1 0 0 1 109.44 278.64 Tm <2E2D466C2E322E20> Tj 1 0 0 1 137.76 278.64 Tm <31332E> Tj 0.72 Tc 1 0 0 1 67.92 264.24 Tm <48416C6463696E656E2C20> Tj 1 0 0 1 115.44 264.00 Tm <532E2C20> Tj 1 0 0 1 128.88 264.00 Tm <4865696E6F6E656E2C20> Tj 1 0 0 1 176.40 263.52 Tm <4D2E2C494772656E6C616D70692C20> Tj 1 0 0 1 248.64 263.04 Tm <532E2C20> Tj 1 0 0 1 262.08 263.04 Tm <4D766B6C71696E656E2C20> Tj 1 0 0 1 313.20 262.80 Tm <482E2C20> Tj 1 0 0 1 329.52 262.56 Tm <527575736B616E656E2C20> Tj 1 0 0 1 381.36 260.40 Tm <4A2E2C20> Tj 1 0 0 1 392.88 262.32 Tm <546F72726F6E656E2C20> Tj 1 0 0 1 438.72 261.84 Tm <522E20> Tj 1 0 0 1 451.44 262.32 Tm <286C396767292E20> Tj 1 0 0 1 486.24 261.60 Tm <53637265656E696E67> Tj 0.48 Tc 1 0 0 1 81.60 249.60 Tm <6F6620> Tj 1 0 0 1 92.88 249.60 Tm <73656C656374656420> Tj 1 0 0 1 128.64 249.36 Tm <666C61766F6E6F69647320> Tj 1 0 0 1 174.48 248.88 Tm <616E6420> Tj 1 0 0 1 192.96 248.64 Tm <7068656E6F6C696320> Tj 1 0 0 1 231.84 248.64 Tm <616369647320> Tj 1 0 0 1 255.36 248.40 Tm <696E20> Tj 1 0 0 1 267.84 248.40 Tm <6C3920> Tj 1 0 0 1 280.08 248.16 Tm <626572726965732E20> Tj 1 0 0 1 313.92 248.16 Tm <466F6F6420> Tj 1 0 0 1 337.44 247.92 Tm <526573656172636820> Tj 1 0 0 1 377.52 247.68 Tm <496E7465726E6174696F6E616C2E20> Tj 1 0 0 1 438.72 247.92 Tm <283332293A20> Tj 1 0 0 1 462.00 246.96 Tm <3334352D3335332E> Tj 0.48 Tc 1 0 0 1 67.68 234.96 Tm <4865696E6F6E656E2C20> Tj 1 0 0 1 116.16 234.72 Tm <492E4D2E2C20> Tj 1 0 0 1 140.64 234.48 Tm <4D6576657220> Tj 1 0 0 1 171.12 234.24 Tm <412E532E20> Tj 1 0 0 1 193.92 234.48 Tm <2832303032292E20> Tj 1 0 0 1 228.72 233.76 Tm <416E74696F786964616E747320> Tj 1 0 0 1 287.28 233.52 Tm <696E20> Tj 1 0 0 1 299.28 233.28 Tm <6672756974732C20> Tj 1 0 0 1 327.84 233.04 Tm <6265727269657320> Tj 1 0 0 1 359.76 233.04 Tm <616E6420> Tj 1 0 0 1 378.96 232.80 Tm <766567657461626C65732E20> Tj 1 0 0 1 428.64 232.56 Tm <496E3A20> Tj 1 0 0 1 444.00 232.56 Tm <467275697420> Tj 1 0 0 1 468.24 232.32 Tm <616E6420> Tj 1 0 0 1 487.20 232.08 Tm <766567657461626C65> Tj 0.72 Tc 1 0 0 1 81.36 219.84 Tm <70726F63657373696E6720> Tj 1 0 0 1 127.92 220.08 Tm <285720> Tj 1 0 0 1 144.48 217.92 Tm <666F6E67656E2C20> Tj 1 0 0 1 178.80 219.36 Tm <65642E292C20> Tj 1 0 0 1 200.40 219.12 Tm <576F6F646865616420> Tj 1 0 0 1 248.88 218.88 Tm <5075626C697368696E6720> Tj 1 0 0 1 295.92 218.64 Tm <4C696D697465642C20> Tj 1 0 0 1 334.08 218.16 Tm <43616D6272696467652C32332D3549> Tj 0.72 Tc 1 0 0 1 67.68 205.44 Tm <4B69686B6F6E656E2C20> Tj 1 0 0 1 115.44 205.20 Tm <4D2E502C20> Tj 1 0 0 1 138.72 205.20 Tm <4865696E416D416B6920> Tj 1 0 0 1 187.20 203.28 Tm <7C2E2C20> Tj 1 0 0 1 197.28 204.72 Tm <4F6C6C696C61696E656E562C20> Tj 1 0 0 1 252.48 204.48 Tm <4865696E6F6E656E20> Tj 1 0 0 1 296.40 204.00 Tm <4D2E20> Tj 1 0 0 1 310.80 204.48 Tm <2832303033292E20> Tj 1 0 0 1 343.92 203.76 Tm <4265727276616E74686F6376616E696E733A69736F6C6174696F6E2C20> Tj 1 0 0 1 470.16 203.04 Tm <6964656E74696669636174696F6E> Tj 0.72 Tc 1 0 0 1 81.36 191.04 Tm <616E6420> Tj 1 0 0 1 100.08 190.80 Tm <616E74696F786964616E7420> Tj 1 0 0 1 150.72 190.80 Tm <616374697669746965732E20> Tj 1 0 0 1 192.96 188.40 Tm <296F75726E616C6F6620> Tj 1 0 0 1 237.60 190.08 Tm <74686520> Tj 1 0 0 1 254.40 189.84 Tm <536369656E636520> Tj 1 0 0 1 288.24 189.60 Tm <6F6620> Tj 1 0 0 1 299.52 189.60 Tm <466F6F6420> Tj 1 0 0 1 323.28 189.36 Tm <616E644167726963756C747572652E20> Tj 1 0 0 1 394.32 189.36 Tm <283833293A20> Tj 1 0 0 1 418.56 188.88 Tm <313430332D6C344974> Tj 0.48 Tc 1 0 0 1 67.44 176.64 Tm <49476C742C20> Tj 1 0 0 1 89.28 176.40 Tm <572C20> Tj 1 0 0 1 105.12 176.40 Tm <466F726E657227272C20> Tj 1 0 0 1 136.80 176.16 Tm <432E452C20> Tj 1 0 0 1 156.96 176.16 Tm <4D617274696E412E2C20> Tj 1 0 0 1 202.56 175.92 Tm <5072696F72522E4C2E20> Tj 1 0 0 1 244.32 175.92 Tm <2849393939292E20> Tj 1 0 0 1 276.96 175.20 Tm <416E74696F786964616E7420> Tj 1 0 0 1 329.28 174.72 Tm <63617061636974762C20> Tj 1 0 0 1 366.24 174.72 Tm <766974616D696E20> Tj 1 0 0 1 400.32 174.48 Tm <432C20> Tj 1 0 0 1 411.60 174.24 Tm <7068656E6F6C69637320> Tj 1 0 0 1 452.88 174.00 Tm <616E6420> Tj 1 0 0 1 470.16 174.00 Tm <616E74686F6379616E696E73> Tj 0.48 Tc 1 0 0 1 81.36 162.00 Tm <616674657220> Tj 1 0 0 1 103.44 162.00 Tm <667265736820> Tj 1 0 0 1 126.72 161.52 Tm <73746F7261676520> Tj 1 0 0 1 158.88 161.28 Tm <6F6620> Tj 1 0 0 1 170.16 161.28 Tm <736D616C6C20> Tj 1 0 0 1 194.88 161.28 Tm <6672756974732E20> Tj 1 0 0 1 222.72 161.04 Tm <2E20> Tj 1 0 0 1 227.52 159.12 Tm <5D6F75726E616C20> Tj 1 0 0 1 261.12 160.56 Tm <6F6620> Tj 1 0 0 1 271.92 160.56 Tm <4167726963756C747572616C20> Tj 1 0 0 1 324.48 160.08 Tm <616E6420> Tj 1 0 0 1 343.20 160.08 Tm <466F6F6420> Tj 1 0 0 1 366.96 159.84 Tm <4368656D69737472792E20> Tj 1 0 0 1 415.68 160.08 Tm <283137293A20> Tj 1 0 0 1 440.40 159.60 Tm <313633382D34363434> Tj 0.72 Tc 1 0 0 1 67.44 147.36 Tm <49286E656B742C20> Tj 1 0 0 1 99.12 146.88 Tm <502C20> Tj 1 0 0 1 111.36 147.12 Tm <4928756D70756C61696E656E2C20> Tj 1 0 0 1 173.76 144.72 Tm <6620> Tj 1 0 0 1 177.84 146.40 Tm <2E2C20> Tj 1 0 0 1 185.52 144.72 Tm <66647276696E656E2C20> Tj 1 0 0 1 226.32 146.16 Tm <522E2C20> Tj 1 0 0 1 241.68 145.92 Tm <52697373616E656E2C20> Tj 1 0 0 1 284.64 145.68 Tm <482E2C20> Tj 1 0 0 1 300.96 145.68 Tm <48656C696F76616172612C20> Tj 1 0 0 1 352.08 145.20 Tm <4D2E2C20> Tj 1 0 0 1 370.08 145.20 Tm <5265756E616E656E2C20> Tj 1 0 0 1 417.36 144.96 Tm <412E2C20> Tj 1 0 0 1 433.44 144.72 Tm <48616B756C696E656E2C20> Tj 1 0 0 1 483.36 144.24 Tm <5420> Tj 1 0 0 1 494.88 144.72 Tm <283230303229> Tj 0.48 Tc 1 0 0 1 81.36 132.48 Tm <466C61766F6E6F696420> Tj 1 0 0 1 125.76 132.24 Tm <696E74616B6520> Tj 1 0 0 1 154.56 132.00 Tm <616E6420> Tj 1 0 0 1 173.04 132.00 Tm <7269736B20> Tj 1 0 0 1 191.04 131.76 Tm <6F6620> Tj 1 0 0 1 202.08 131.52 Tm <6368726F6E696320> Tj 1 0 0 1 235.92 131.28 Tm <64697365617365732E20> Tj 1 0 0 1 274.08 131.04 Tm <416D65726963616E20> Tj 1 0 0 1 317.28 128.88 Tm <6C6F75726E616C20> Tj 1 0 0 1 350.88 130.56 Tm <6F6620> Tj 1 0 0 1 362.16 130.32 Tm <436C696E6963616C20> Tj 1 0 0 1 397.20 130.32 Tm <4E7574726974696F6E2E20> Tj 1 0 0 1 443.52 130.56 Tm <283736293A20> Tj 1 0 0 1 466.32 129.60 Tm <3536302D353638> Tj 0.72 Tc 1 0 0 1 67.44 118.08 Tm <4D65657474652D52696968696E656E2C20> Tj 1 0 0 1 144.24 117.60 Tm <4928522E2C20> Tj 1 0 0 1 170.40 117.36 Tm <49476D616C2D456C64696E2C20> Tj 1 0 0 1 229.44 116.88 Tm <412E2C20> Tj 1 0 0 1 247.20 116.64 Tm <4D617474696C612C20> Tj 1 0 0 1 285.60 116.40 Tm <50482E2C20> Tj 1 0 0 1 310.08 116.16 Tm <476F6E7A646C657A2D506172616D64732C20> Tj 1 0 0 1 393.84 115.92 Tm <412E4D2E2C20> Tj 1 0 0 1 423.12 115.68 Tm <546F72726F6E656E2C20> Tj 1 0 0 1 469.68 115.20 Tm <412E522E20> Tj 1 0 0 1 494.64 115.68 Tm <2832303031292E> Tj 0.48 Tc 1 0 0 1 81.36 103.44 Tm <446973747269627574696F6E20> Tj 1 0 0 1 138.24 103.20 Tm <616E6420> Tj 1 0 0 1 158.88 103.20 Tm <636F6E74656E7420> Tj 1 0 0 1 196.32 102.72 Tm <6F6620> Tj 1 0 0 1 209.52 102.48 Tm <7068656E6F6C696320> Tj 1 0 0 1 250.56 102.24 Tm <636F6D706F756E647320> Tj 1 0 0 1 304.56 102.00 Tm <696E20> Tj 1 0 0 1 317.76 101.76 Tm <656967687465656E20> Tj 1 0 0 1 358.56 101.52 Tm <7363616E64696E617669616E20> Tj 1 0 0 1 417.84 101.04 Tm <626572727620> Tj 1 0 0 1 445.68 101.04 Tm <737065636965732E20> Tj 1 0 0 1 481.92 98.88 Tm <666F75726E616C20> Tj 1 0 0 1 517.68 100.32 Tm <6F66> Tj 0.48 Tc 1 0 0 1 80.40 89.04 Tm <4167726963756C747572616C20> Tj 1 0 0 1 133.44 88.56 Tm <616E6420> Tj 1 0 0 1 151.92 88.56 Tm <466F6F6420> Tj 1 0 0 1 175.68 88.08 Tm <4368656D697374727620> Tj 1 0 0 1 224.40 88.32 Tm <283532293A20> Tj 1 0 0 1 247.68 87.60 Tm <34343720> Tj 1 0 0 1 264.72 87.60 Tm <3720> Tj 1 0 0 1 271.20 89.52 Tm <2D34313836> Tj 0.96 Tc /F3 10.0 Tf 1 0 0 1 38.64 54.96 Tm <363336> Tj 0.96 Tc /F3 14.0 Tf 1 0 0 1 278.88 47.76 Tm <4920> Tj 1 0 0 1 284.16 48.96 Tm <343B2220> Tj 1 0 0 1 301.20 48.72 Tm <696C6674562669735D7B6920> Tj 1 0 0 1 345.84 48.72 Tm <4920> Tj 1 0 0 1 351.12 48.48 Tm <3A2220> Tj 1 0 0 1 362.16 48.48 Tm <4927745B5B7D756841522A6E7A757420> Tj 1 0 0 1 432.00 47.76 Tm <24666C6C7D2A3B6C5D41696C522A662A2A746C6C41> Tj ET endstream endobj 31 0 obj 22025 endobj 32 0 obj << /Length 33 0 R >> stream ConclusionsSour cherrv and red currant have considerablv lower anlount of pollphenols and anthocvanins and showlower antioxidant activitv in comparison to blueberry, elderberrv and black currant which are verv rich in thesePhrtochemicals and possess higher antioxidant activitv against DPPH radical. There are marked differencesin the phenolic profiles of investigated fruits. Elderberry and blueberrv yere characterized bv high portionof quercetin among the phenolic compounds studied. In black currant, flavonols and hvdroxvcinnamic acidsr,vere relativelv equallv distributed. P-hydrowbenzoic acid was the main phenolic compound of red currant. Insour cherrl', p-coumaric and caffeic acid lvere the rlrost abundant phenolic compounds. According to data onpolvphenol content and antioxidant activitv of investigated fruits, blueberrv eiderberrv and black currant canbe regarded as go<-rd candidates in production of health beneficial functional foods.Thble 2. Percentage distribution of flavonols and phenolic acids of fruits Fruits Hvdroxvbenzoicacids Hvdroxvcinnamic acids Flavonols Total p-Hy-droxv- Ellagicbenzoic acidacid o/oo/o P-co."- Ferulicmanc . raclo"i.| o/o Mvric- Querce- IGemp-etin tin ferol Caffeicacido/o BlueberrvElderberrvBlack cur-rantRed cur-rantSourcherrv 5.3 r r 2.0810.r013.57B.0s30.83 t7.957.2521.026.4051.79 2.034.17 15.83J/.)+3.87 5 t.B3B 1.48r5.BIt7.lB15.55 0.28 100.001.r7 100.002.28 100.000.76 r00.00l.83 100.00 63.71 ReferencesBeattie 1., Crozter A., Duthie G. (2005). Potential health benefits of berries. Current Nutrition and FoodScience (l):71-86Benvenuti, S., Pellati, F., Melegari, M., Bertelli, D. (2004). Polvphenols, anthocvanins, ascorbic acid, arrdradical scavenging activitv of Rubus, Ribes, and Aronia. lournal of Food Science (69): I 64-169Giusti, M.M., Wrolstad, R.8., (2001). Anthocvanins. Characterization and measurement rvith UV-visiblespectroscopy. Irr: Current protocols in food analr.tical chemistrv (R.E. Wrolstad ed), Wilev, Nerv York,Fl.2.1 .-Fl.2. 13.HAldcinen, S., Heinonen, M.,IGrenlampi, S., Mvklqinen, H., Ruuskanen, J., Torronen, R. (l9gg). Screeningof selected flavonoids and phenolic acids in l9 berries. Food Research International. (32): 345-353.Heinonen, I.M., Mever A.S. (2002). Antioxidants in fruits, berries and vegetables. In: Fruit and vegetableprocessing (W fongen, ed.), Woodhead Publishing Limited, Cambridge,23-5IKihkonen, M.P, HeinAmAki |., OllilainenV, Heinonen M. (2003). Berrvanthocvanins:isolation, identificationand antioxidant activities. )ournalof the Science of Food andAgriculture. (83): 1403-l4ItIGlt, W, Forner'', C.E, MartinA., PriorR.L. (I999). Antioxidant capacitv, vitamin C, phenolics and anthocyaninsafter fresh storage of small fruits. . ]ournal of Agricultural and Food Chemistry. (17): 1638-4644I(nekt, P, I(umpulainen, f ., fdrvinen, R., Rissanen, H., Heliovaara, M., Reunanen, A., Hakulinen, T (2002)Flavonoid intake and risk of chronic diseases. American lournal of Clinical Nutrition. (76): 560-568Meette-Riihinen, I(R., IGmal-Eldin, A., Mattila, PH., Gonzdlez-Paramds, A.M., Torronen, A.R. 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199.92 53.04 Tm <6C6C35692C4A20> Tj 1 0 0 1 225.36 50.64 Tm <55275D6927692C6C2C74667220> Tj 1 0 0 1 267.36 50.88 Tm <6C743B20> Tj 1 0 0 1 281.76 50.40 Tm <4C697420> Tj 1 0 0 1 296.64 50.16 Tm <497420> Tj 1 0 0 1 312.48 49.92 Tm <69> Tj 0.96 Tc /F3 10.0 Tf 1 0 0 1 498.24 53.28 Tm <363337> Tj ET endstream endobj 39 0 obj 7989 endobj 40 0 obj << /Length 41 0 R >> stream Waterhouse A (Ma,v, lOth 2006). http://waterhouse.ucdavis.edu/phenoVfolinmicro.htmZadernorvski, R., Naczk, M., Nesterowicz,I. Q005). Phenolic acids in son-re smallberries. fournal ofAgriculturaland Food Chemistm (53): 2llB-2124. Antioksidacijska aktivnost, flavonoli i fenolne kiseline razliditih vrsta vo6a SaietakUkupni polifenoli (TP), ukupni antociianini (TA) i antioksidacijska aktivnost razlititog vo6a (crni i crveni ribiz,vi5nja, bobice bazge, borovnica) odredeni su Folin-Ciocalteau, pH diferencijalnom i DPPH metodom. Da bi seidentificirali pojedini neantociianinski fenolni spoievi prisutni u izabranom vo6u [flavonoli (kvercetin, miricetin,kaempferol), fenolne kiseline (p-kumarinska, kafeinska, feruliina, p-hidroksibenzojeva i elaginska kiselina)],primjenjena je HPLC metoda. Najveie koliiine TP i TA te najjade antioksidaciiske aktivnosti pronadene su uborormici, bobicama bazge i crnom ribiziu. Glar'na neantocijaninska fenolna komponenta bazge i borovnice jekvercetin. U crnom ribizlu ie miricetin najrasprostranjeniji fenolni spol, p-hidroksibenzojeva ldselina je glar,nafenolna komponenta crvenog ribizla, dok su u vi5nji najrasprostranienije kafeinsha i p-kumarinska kiselina.Kljuine rijeii: antocijanini, bobidasto voce, fenolne kiseline, flavonoli : :'; iln0A'i!Ai! & ::: I i,lTlRLiiTill!AL $Yl11 ll5i,J U']i'i,l,tfr lt; Lit It i 637 endstream endobj 41 0 obj 1356 endobj 42 0 obj << /Length 27 >> stream % CANON_PFINF_TYPE0_TEXTON endstream endobj 43 0 obj << /Length 45 >> stream q 597.12 0 0 835.20 0.00 0.00 cm /Obj37 Do Q endstream endobj 44 0 obj << /Type /Page /MediaBox [ 0 0 597.12 835.20 ] /Parent 11 0 R /Resources << /Font << /F3 5 0 R >> /XObject << /Obj37 37 0 R >> /Subtype 40 0 R /ProcSet [ /PDF /Text /ImageB /ImageC /ImageI ] >> /Contents [ 42 0 R 43 0 R 38 0 R ] >> endobj 45 0 obj << /Type /XObject /Subtype /Image /Width 2488 /Height 3480 /BitsPerComponent 1 /ColorSpace /DeviceGray /Filter /CCITTFaxDecode /DecodeParms << /K -1 /Columns 2488 >> /Length 26238 >> stream -15e&D-Q?޾ Dt̀Х*g]L0piM4;9wFdEL, :t&+rΐ3UuA<'t!g juˊRXZCS2xe0H! 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