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Pregled bibliografske jedinice broj: 1177931

Multi-faceted reactivity of N- fluorobenzenesulfonimide (NFSI) under mechanochemical conditions: fluorination, fluorodemethylation, sulfonylation, and amidation reactions

Hernández, José G.; Ardila-Fierro, Karen J.; Barišić, Dajana; Geneste, Hervé
Multi-faceted reactivity of N- fluorobenzenesulfonimide (NFSI) under mechanochemical conditions: fluorination, fluorodemethylation, sulfonylation, and amidation reactions // Beilstein journal of organic chemistry, 18 (2022), 182-189 doi:10.3762/bjoc.18.20 (međunarodna recenzija, članak, znanstveni)

CROSBI ID: 1177931 Za ispravke kontaktirajte CROSBI podršku putem web obrasca

Naslov
Multi-faceted reactivity of N- fluorobenzenesulfonimide (NFSI) under mechanochemical conditions: fluorination, fluorodemethylation, sulfonylation, and amidation reactions

Autori
Hernández, José G. ; Ardila-Fierro, Karen J. ; Barišić, Dajana ; Geneste, Hervé

Izvornik
Beilstein journal of organic chemistry (2195-951X) 18 (2022); 182-189

Vrsta, podvrsta i kategorija rada
Radovi u časopisima, članak, znanstveni

Ključne riječi
amidation ; ball mill ; fluorination ; in situ monitoring ; mechanochemistry ; NFSI ; Raman monitoring ; sulfonylation

Sažetak
In the search for versatile reagents compatible with mechanochemical techniques, in this work we studied the reactivity of N- fluorobenzenesulfonimide (NFSI) by ball milling. We corroborated that, by mechanochemistry, NFSI can engage in a variety of reactions such as fluorinations, fluorodemethylations, sulfonylations, and amidations. In comparison to the protocols reported in solution, the mechanochemical reactions were accomplished in the absence of solvents, in short reaction times, and in yields comparable to or higher than their solvent-based counterparts.

Izvorni jezik
Engleski

Znanstvena područja
Kemija



POVEZANOST RADA

Projekti:
HRZZ-IP-2019-04-9951 - Mehanokemijska aktivacija i funkcionalizacija veze C–H potaknuta paladijem i usmjerena ligandom (MECHEMFUN) (Ćurić, Manda, HRZZ ) ( CroRIS)

Ustanove:
Institut "Ruđer Bošković", Zagreb

Profili:

Avatar Url Dajana Barišić (autor)

Poveznice na cjeloviti tekst rada:

Pristup cjelovitom tekstu rada doi www.beilstein-journals.org doi.org fulir.irb.hr

Citiraj ovu publikaciju:

Hernández, José G.; Ardila-Fierro, Karen J.; Barišić, Dajana; Geneste, Hervé
Multi-faceted reactivity of N- fluorobenzenesulfonimide (NFSI) under mechanochemical conditions: fluorination, fluorodemethylation, sulfonylation, and amidation reactions // Beilstein journal of organic chemistry, 18 (2022), 182-189 doi:10.3762/bjoc.18.20 (međunarodna recenzija, članak, znanstveni)
Hernández, J., Ardila-Fierro, K., Barišić, D. & Geneste, H. (2022) Multi-faceted reactivity of N- fluorobenzenesulfonimide (NFSI) under mechanochemical conditions: fluorination, fluorodemethylation, sulfonylation, and amidation reactions. Beilstein journal of organic chemistry, 18, 182-189 doi:10.3762/bjoc.18.20.
@article{article, author = {Hern\'{a}ndez, Jos\'{e} G. and Ardila-Fierro, Karen J. and Bari\v{s}i\'{c}, Dajana and Geneste, Herv\'{e}}, year = {2022}, pages = {182-189}, DOI = {10.3762/bjoc.18.20}, keywords = {amidation, ball mill, fluorination, in situ monitoring, mechanochemistry, NFSI, Raman monitoring, sulfonylation}, journal = {Beilstein journal of organic chemistry}, doi = {10.3762/bjoc.18.20}, volume = {18}, issn = {2195-951X}, title = {Multi-faceted reactivity of N- fluorobenzenesulfonimide (NFSI) under mechanochemical conditions: fluorination, fluorodemethylation, sulfonylation, and amidation reactions}, keyword = {amidation, ball mill, fluorination, in situ monitoring, mechanochemistry, NFSI, Raman monitoring, sulfonylation} }
@article{article, author = {Hern\'{a}ndez, Jos\'{e} G. and Ardila-Fierro, Karen J. and Bari\v{s}i\'{c}, Dajana and Geneste, Herv\'{e}}, year = {2022}, pages = {182-189}, DOI = {10.3762/bjoc.18.20}, keywords = {amidation, ball mill, fluorination, in situ monitoring, mechanochemistry, NFSI, Raman monitoring, sulfonylation}, journal = {Beilstein journal of organic chemistry}, doi = {10.3762/bjoc.18.20}, volume = {18}, issn = {2195-951X}, title = {Multi-faceted reactivity of N- fluorobenzenesulfonimide (NFSI) under mechanochemical conditions: fluorination, fluorodemethylation, sulfonylation, and amidation reactions}, keyword = {amidation, ball mill, fluorination, in situ monitoring, mechanochemistry, NFSI, Raman monitoring, sulfonylation} }

Časopis indeksira:


  • Current Contents Connect (CCC)
  • Web of Science Core Collection (WoSCC)
    • Science Citation Index Expanded (SCI-EXP)
    • SCI-EXP, SSCI i/ili A&HCI
  • Scopus

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