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Poisson-Boltzmann approach for sterically asymmetric electrolytes (CROSBI ID 593088)

Prilog sa skupa u zborniku | sažetak izlaganja sa skupa

Popović, Marko ; Šiber, Antonio Poisson-Boltzmann approach for sterically asymmetric electrolytes // 7th Christmas Biophysics Workshop : Book of Abstracts / Pabst, Georg ; Heftberger, Peter ; Kollmitzer, Benjamin (ur.). Graz, 2012. str. 6-6

Podaci o odgovornosti

Popović, Marko ; Šiber, Antonio

engleski

Poisson-Boltzmann approach for sterically asymmetric electrolytes

We derive a modification of the Poisson-Boltzmann equation considering steric effects of different size ions. Our equation represents a generalization of previous work for equal size ions [I. Borukhov, D. Andelman and H. Orland, Phys. Rev. Lett. 79, 435 (1997)] and allows more general calculations. We show that proposed modification predicts asymmetry of the double-layer differential capacitance. Our derivation provides analytical framework for previously proposed heuristic modification of the Poisson-Boltzmann equation, which also predicts the same effect [A.A. Kornyshev, J. Phys. Chem. B 111, 5545 (2007)].

poisson-boltzmann; electrostatics; ions

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Podaci o prilogu

6-6.

2012.

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objavljeno

Podaci o matičnoj publikaciji

7th Christmas Biophysics Workshop : Book of Abstracts

Pabst, Georg ; Heftberger, Peter ; Kollmitzer, Benjamin

Graz:

Podaci o skupu

7th Christmas Biophysics Workshop (XBW 2012)

predavanje

17.12.2012-18.12.2012

Riegersburg, austrija

Povezanost rada

Fizika