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Low-temperature thermodynamic investigation of the sulphur organic salts (TMTTF)(2)PF6 and (TMTTF)(2)Br (TMTTF = tetramethyltetrathiafulvalene): II. Dynamical aspects


Lasjaunias, Jean-Claude; Monceau, Pierre; Starešinić, Damir; Biljaković, Katica; Carcel, C.; Fabre, J.M.
Low-temperature thermodynamic investigation of the sulphur organic salts (TMTTF)(2)PF6 and (TMTTF)(2)Br (TMTTF = tetramethyltetrathiafulvalene): II. Dynamical aspects // Journal of physics. Condensed matter, 14 (2002), 36; 8583-8594 (međunarodna recenzija, članak, znanstveni)


Naslov
Low-temperature thermodynamic investigation of the sulphur organic salts (TMTTF)(2)PF6 and (TMTTF)(2)Br (TMTTF = tetramethyltetrathiafulvalene): II. Dynamical aspects

Autori
Lasjaunias, Jean-Claude ; Monceau, Pierre ; Starešinić, Damir ; Biljaković, Katica ; Carcel, C. ; Fabre, J.M.

Izvornik
Journal of physics. Condensed matter (0953-8984) 14 (2002), 36; 8583-8594

Vrsta, podvrsta i kategorija rada
Radovi u časopisima, članak, znanstveni

Ključne riječi
Density-wave systems; phase-transitions; glass-transition; spin-glasses; specific heat; relaxations

Sažetak
This contribution is in continuation of our preceding publication (Lasjaunias J C, Brison J P, Monceau P, Staresinic D, Biljakovic K, Carcel C and Fabre J M 2002 J. Phys.: Condens. Matter 14 837) in which we have considered general aspects of the low-temperature thermodynamical properties of the quasi-one-dimensional organic salts based on sulphur donors with different ground states: (TMTTF)(2)PF6 in the spin-Peierls state and (TMTTF)(2)Br (TMTTF = tetramethyltetrathiafulvalene) with commensurate spin modulation. In this part, part 11, we present our results on the dynamical aspects related to the non-equilibrium phenomena measured below I K. The metastable states excited to slightly higher temperature (by only a few per cent of the starting T-0) relax very slowly to the heat bath environment, depending on the duration of the heat pumping. We compare the features observed in the relaxation rates in these two sulphur compounds with those measured for the incommensurate spin-density-wave compound (TMTSF)(2)PF6. We discuss the possible nature of the long-living low-energy excitations lying at the origin of this complex dynamical behaviour, in relation to their ground states.

Izvorni jezik
Engleski

Znanstvena područja
Fizika



POVEZANOST RADA


Projekt / tema
0035014

Ustanove
Institut za fiziku, Zagreb

Časopis indeksira:


  • Current Contents Connect (CCC)
  • Web of Science Core Collection (WoSCC)
    • Science Citation Index Expanded (SCI-EXP)
    • SCI-EXP, SSCI i/ili A&HCI
  • Scopus